Volatile organic compounds (VOCs) during non-haze and haze days in Shanghai: characterization and secondary organic aerosol (SOA) formation

2017 ◽  
Vol 24 (22) ◽  
pp. 18619-18629 ◽  
Author(s):  
Deming Han ◽  
Zhen Wang ◽  
Jinping Cheng ◽  
Qian Wang ◽  
Xiaojia Chen ◽  
...  
Keyword(s):  
Volatile Organic Compounds ◽  
Organic Compounds ◽  
Secondary Organic Aerosol ◽  
Organic Aerosol ◽  
Volatile Organic ◽  
Haze Days

scholarly journals Aging of atmospheric aerosols and the role of iron in catalyzing brown carbon formation

2021 ◽  
Author(s):  
Hind A. A. Al-Abadleh
Keyword(s):  
Volatile Organic Compounds ◽  
Organic Compounds ◽  
Atmospheric Aerosols ◽  
Secondary Organic Aerosol ◽  
Organic Aerosol ◽  
Atmospheric Oxidation ◽  
Carbon Formation ◽  
Brown Carbon ◽  
Volatile Organic

Extensive research has been done on the processes that lead to the formation of secondary organic aerosol (SOA) including atmospheric oxidation of volatile organic compounds (VOCs) from biogenic and anthropogenic...

scholarly journals Secondary organic aerosol enhanced by increasing atmospheric oxidizing capacity in Beijing–Tianjin–Hebei (BTH), China

2019 ◽  
Vol 19 (11) ◽  
pp. 7429-7443 ◽  
Author(s):  
Tian Feng ◽  
Shuyu Zhao ◽  
Naifang Bei ◽  
Jiarui Wu ◽  
Suixin Liu ◽  
...  
Keyword(s):  
Air Pollution ◽  
Volatile Organic Compounds ◽  
Organic Compounds ◽  
Secondary Organic Aerosol ◽  
Action Plan ◽  
Spatial Relationship ◽  
Pollution Prevention ◽  
Organic Aerosol ◽  
Temporal Variations ◽  
Volatile Organic

Abstract. The implementation of the Air Pollution Prevention and Control Action Plan in China since 2013 has profoundly altered the ambient pollutants in the Beijing–Tianjin–Hebei (BTH) region. Here we show observations of substantially increased O3 concentrations (about 30 %) and a remarkable increase in the ratio of organic carbon (OC) to elemental carbon (EC) in BTH during the autumn from 2013 to 2015, revealing an enhancement in atmospheric oxidizing capacity (AOC) and secondary organic aerosol (SOA) formation. To explore the impacts of increasing AOC on the SOA formation, a severe air pollution episode from 3 to 8 October 2015 with high O3 and PM2.5 concentrations is simulated using the WRF-Chem model. The model performs reasonably well in simulating the spatial distributions of PM2.5 and O3 concentrations over BTH and the temporal variations in PM2.5, O3, NO2, OC, and EC concentrations in Beijing compared to measurements. Sensitivity studies show that the change in AOC substantially influences the SOA formation in BTH. A sensitivity case characterized by a 31 % O3 decrease (or 36 % OH decrease) reduces the SOA level by about 30 % and the SOA fraction in total organic aerosol by 17 % (from 0.52 to 0.43, dimensionless). Spatially, the SOA decrease caused by reduced AOC is ubiquitous in BTH, but the spatial relationship between SOA concentrations and the AOC is dependent on the SOA precursor distribution. Studies on SOA formation pathways further show that when the AOC is reduced, the SOA from oxidation and partitioning of semivolatile primary organic aerosol (POA) and co-emitted intermediate volatile organic compounds (IVOCs) decreases remarkably, followed by those from anthropogenic and biogenic volatile organic compounds (VOCs). Meanwhile, the SOA decrease in the irreversible uptake of glyoxal and methylglyoxal on the aerosol surfaces is negligible.

Emission of volatile organic compounds and production of secondary organic aerosol from stir-frying spices

2017 ◽  
Vol 599-600 ◽  
pp. 1614-1621 ◽  
Author(s):  
Tengyu Liu ◽  
Qianyun Liu ◽  
Zijun Li ◽  
Lei Huo ◽  
ManNin Chan ◽  
...  
Keyword(s):  
Volatile Organic Compounds ◽  
Organic Compounds ◽  
Secondary Organic Aerosol ◽  
Organic Aerosol ◽  
Volatile Organic

scholarly journals Emissions of Volatile Organic Compounds (VOCs) from an Open-Circuit Dry Cleaning Machine Using a Petroleum-Based Organic Solvent: Implications for Impacts on Air Quality

Atmosphere ◽  
2021 ◽  
Vol 12 (5) ◽  
pp. 637
Author(s):  
Hyeonji Lee ◽  
Kyunghoon Kim ◽  
Yelim Choi ◽  
Daekeun Kim
Keyword(s):  
Air Quality ◽  
Volatile Organic Compounds ◽  
Organic Compounds ◽  
Organic Solvents ◽  
Secondary Organic Aerosol ◽  
Organic Aerosol ◽  
Tropospheric Chemistry ◽  
Dry Cleaning ◽  
Volatile Organic ◽  
Vocs Emission

Volatile organic compounds (VOCs) are known to play an important role in tropospheric chemistry, contributing to ozone and secondary organic aerosol (SOA) generation. Laundry facilities, using petroleum-based organic solvents, are one of the sources of VOCs emissions. However, little is known about the significance of VOCs, emitted from laundry facilities, in the ozone and SOA generation. In this study, we characterized VOCs emission from a dry-cleaning process using petroleum-based organic solvents. We also assessed the impact of the VOCs on air quality by using photochemical ozone creation potential and secondary organic aerosol potential. Among 94 targeted compounds including toxic organic air pollutants and ozone precursors, 36 compounds were identified in the exhaust gas from a drying machine. The mass emitted from one cycle of drying operation (40 min) was the highest in decane (2.04 g/dry cleaning). Decane, nonane, and n-undecane were the three main contributors to ozone generation (more than 70% of the total generation). N-undecane, decane, and n-dodecane were the three main contributors to the SOA generation (more than 80% of the total generation). These results help to understand VOCs emission from laundry facilities and impacts on air quality.

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