In-situ sunlight-driven tuning of photo-induced electron-hole generation and separation rates in bismuth oxychlorobromide for highly efficient water decontamination under visible light irradiation

Author(s):  
Amani M. Alansi ◽  
Talal F. Qahtan ◽  
N. Al Abass ◽  
Maha Al-Qunaibit ◽  
Tawfik A. Saleh
Nanoscale ◽  
2017 ◽  
Vol 9 (38) ◽  
pp. 14423-14430 ◽  
Author(s):  
Zheguan Lin ◽  
Jinjin Lin ◽  
Lingting Huang ◽  
Xiaoyan Zhang ◽  
Ying Wang ◽  
...  

Constructing a heterojunction on the MnSb2S4 of a sandwich structure ([SbS]+–[MnS2]2−–[SbS]+) is more favorable to the separation of photogenerated charge to improve photocatalytic activity.


RSC Advances ◽  
2021 ◽  
Vol 11 (33) ◽  
pp. 20446-20456
Author(s):  
Xi Ma ◽  
Ziwei Wang ◽  
Haoguo Yang ◽  
Yiqiu Zhang ◽  
Zizhong Zhang ◽  
...  

Compared with traditional layered graphene, graphene hydrogels have been used to construct highly efficient visible light-excited photocatalysts due to their particular three-dimensional network structure and efficient electron transport capacity.


2020 ◽  
Vol 10 (6) ◽  
pp. 1609-1618 ◽  
Author(s):  
Chao Zhang ◽  
Jiandong Liu ◽  
Xingliang Liu ◽  
Shiai Xu

Reaction mechanism for the higher photocatalytic performance of H2 production of g-C3N4NSs/TC1 under visible light irradiation (λ ≥ 400 nm).


2015 ◽  
Vol 2015 ◽  
pp. 1-12 ◽  
Author(s):  
Xiangchao Meng ◽  
Zisheng Zhang

In photocatalysis, the recombination of electron-hole pairs is generally regarded as one of its most serious drawbacks. The synthesis of various composites with heterojunction structures has increasingly shed light on preventing this recombination. In this work, a BiOBr-Bi2WO6photocatalytic heterojunction semiconductor was synthesized by the facile hydrothermal method and applied in the photocatalytic degradation process. It was determined that both reaction time and temperature significantly affected the crystal structure and morphologies of the photocatalysts. BiOBr (50 at%)-Bi2WO6composites were prepared under optimum synthesis conditions (120°C for 6 h) and by theoretically analyzing the DRS results, it was determined that they possessed the suitable band gap (2.61 eV) to be stimulated by visible-light irradiation. The photocatalytic activities of the as-prepared photocatalysts were evaluated by the degradation ofRhodamine B (RhB)under visible-light irradiation. The experimental conditions, including initial concentration, pH, and catalyst dosage, were explored and the photocatalysts in this system were proven stable enough to be reused for several runs. Moreover, the interpreted mechanism of the heterojunction enhancement effect proved that the synthesis of a heterojunction structure provided an effective method to decrease the recombination rate of the electron-hole pairs, thereby improving the photocatalytic activity.


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