scholarly journals Radiation Effects Issues Related to U.S. Doe Site Remediation and Nuclear Waste Storage

1994 ◽  
Vol 353 ◽  
Author(s):  
William J. Weber ◽  
Rodney C. Ewing

AbstractSite restoration activities at DOE facilities and the permanent disposal of nuclear waste generated at the same DOE facilities involve working with and within various types and levels of radiation fields. Radionuclide decay and the associated radiation fields lead to physical and chemical changes that can degrade or enhance material properties. This paper reviews the impact of radiation fields on site restoration activities and on the release rate of radionuclides to the biosphere from nuclear waste forms.

1981 ◽  
Vol 11 ◽  
Author(s):  
J.W. Wald ◽  
P. Offemann

Radiation effects studies in both glass and glass ceramic nuclear waste forms have identified a rare-earth titanate phase of the general formula (RE) 2Ti207 which is capable of acting as a host phase for actinides.1,2 Ringwood and co-workers3 have also proposed a structurally similar phase, zirconolite (CaZrTi2 07), as one of the primary host phases in the SYNROC waste form. Data from these and other previous studies, as well as mineralogical information available on these titanate phases, have not provided an unambiguous interpretation of the effects of radiation damage relative to nuclear waste forms. This paper reports new laboratory data concerning radiation damage effects in both of these phases.


1981 ◽  
Vol 6 ◽  
Author(s):  
Paul G. Huray ◽  
M. T. Spaar ◽  
S. E. Nave ◽  
J. M. Legan ◽  
L. A. Boatner ◽  
...  

The electronic charge states and site symmetries of the radioactive ions incorporated in nuclear waste forms are of considerable importance in determining the physical and chemical properties of these materials. An in situ characterization of these ions is, unfortunately, often difficult – especially when a mixture of charge states and local crystal symmetries exist. The application of Mbssbauer spectroscopy represents a powerful technique for obtaining solid state chemical information.


2021 ◽  
pp. 0958305X2110513
Author(s):  
Adam J. Mallette ◽  
Aparajita Datta ◽  
Ramanan Krishnamoorti

Over the last 50 years, nuclear energy has reduced US energy-related CO2 emissions by over 30 gigatons compared to if the same electricity were produced by fossil fuels such as coal and natural gas. However, many kilotons of spent nuclear fuel have accumulated at different sites across the country, and sociopolitical factors have frustrated efforts to address the challenge of nuclear waste disposal. Presently, a consolidated interim storage facility in Andrews, Texas, provides a promising temporary solution. In this paper, we compare the technical and policy risks of the project to continued storage at independent spent fuel storage installations. Our results indicate that the cost of the radiological risk is low (<$30,000) for both scenarios. However, policy and societal considerations will impact the viability of the proposed consolidated interim storage facility. The safety and suitability of this interim storage facility will be affected by when a permanent repository becomes available, whether insurance for offsite waste storage is available, and the impact of climate risks. Although a consolidated interim storage facility at Andrews can potentially serve as a safe and economically advantageous solution, we highlight why these concerns must be addressed for the successful implementation of this facility, and more broadly for the future of the US nuclear industry.


1983 ◽  
Vol 60 (2) ◽  
pp. 178-198 ◽  
Author(s):  
William J. Weber ◽  
Frank P. Roberts

1982 ◽  
Vol 15 ◽  
Author(s):  
William J. Weber

ABSTRACTThe current status of radiation effects in solid nuclear waste forms is reviewed. The general nature of radiation effects and the simulation techniques used are briefly discussed. Recently reported data on radiation effects are presented and discussed, and those areas requiring further theoretical or experimental study are identified.


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