scholarly journals Aerosol-radiation feedback deteriorates the wintertime haze in North China Plain

2019 ◽  
Author(s):  
Jiarui Wu ◽  
Naifang Bei ◽  
Bo Hu ◽  
Suixin Liu ◽  
Meng Zhou ◽  
...  
Keyword(s):  
Solar Radiation ◽  
Air Pollutants ◽  
North China Plain ◽  
North China ◽  
Radiative Properties ◽  
Surface Cooling ◽  
Near Surface ◽  
Incoming Solar Radiation ◽  
Haze Pollution ◽  
Pm2.5 Concentration

Abstract. Atmospheric aerosols or fine particulate matters (PM2.5) scatter or absorb a fraction of the incoming solar radiation to cool or warm the atmosphere, decreasing surface temperature and altering atmospheric stability to further affect the dispersion of air pollutants in the planetary boundary layer (PBL). In the present study, simulations during a persistent and heavy haze pollution episode from 05 December 2015 to 04 January 2016 in the North China Plain (NCP) were performed using the WRF-CHEM model to comprehensively quantify contributions of the aerosol shortwave radiative feedback (ARF) to near-surface PM2.5 mass concentrations. The WRF-CHEM model generally performs well in simulating the temporal variations and spatial distributions of air pollutants concentrations compared to observations at ambient monitoring sites in NCP, and the simulated diurnal variations of aerosol species are also consistent with the measurements in Beijing. Additionally, the model simulates well the aerosol radiative properties, the downward shortwave flux, and the PBL height against observations in NCP during the episode. During the episode, the ARF deteriorates the haze pollution, increasing the near-surface PM2.5 concentration in NCP by 10.2 μg m−3 or with a contribution of 7.8 %. Sensitivity studies have revealed that high loadings of PM2.5 during the episode attenuate the incoming solar radiation down to the surface, cooling the temperature of the low-level atmosphere to suppress development of PBL and decrease the surface wind speed, further enhancing the relative humidity and hindering the PM2.5 dispersion and consequently exacerbating the haze pollution in NCP. The ensemble analysis indicates that when the near-surface PM2.5 mass concentration increases from around 50 to several hundred μg m−3, the ARF contributes to the near-surface PM2.5 by more than 20 % during daytime in NCP, substantially aggravating the heavy haze formation. However, when the near-surface PM2.5 concentration is less than around 50 μg m−3, the ARF generally reduces the near-surface PM2.5 concentration due to the consequent perturbation of atmospheric dynamic fields.

scholarly journals Aerosol–radiation feedback deteriorates the wintertime haze in the North China Plain

2019 ◽  
Vol 19 (13) ◽  
pp. 8703-8719 ◽  
Author(s):  
Jiarui Wu ◽  
Naifang Bei ◽  
Bo Hu ◽  
Suixin Liu ◽  
Meng Zhou ◽  
...  
Keyword(s):  
Solar Radiation ◽  
Air Pollutants ◽  
North China Plain ◽  
North China ◽  
Near Surface ◽  
The North ◽  
The North China Plain ◽  
Incoming Solar Radiation ◽  
Haze Pollution ◽  
Pm2.5 Concentration

Abstract. Atmospheric aerosols scatter or absorb a fraction of the incoming solar radiation to cool or warm the atmosphere, decreasing surface temperature and altering atmospheric stability to further affect the dispersion of air pollutants in the planetary boundary layer (PBL). In the present study, simulations during a persistent and heavy haze pollution episode from 5 December 2015 to 4 January 2016 in the North China Plain (NCP) were performed using the Weather Research and Forecasting model with Chemistry (WRF-Chem) to comprehensively quantify contributions of aerosol shortwave radiative feedback (ARF) to near-surface (around 15 m above the ground surface) PM2.5 mass concentrations. The WRF-Chem model generally performs well in simulating the temporal variations and spatial distributions of air pollutants concentrations compared to observations at ambient monitoring sites in the NCP, and the simulated diurnal variations of aerosol species are also consistent with the measurements in Beijing. Additionally, the model simulates the aerosol radiative properties, the downward shortwave flux, and the PBL height against observations in the NCP well. During the episode, ARF deteriorates the haze pollution, increasing the near-surface PM2.5 concentrations in the NCP by 10.2 µg m−3 or with a contribution of 7.8 % on average. Sensitivity studies have revealed that high loadings of PM2.5 attenuate the incoming solar radiation reaching the surface to cool the low-level atmosphere, suppressing the development of the PBL, decreasing the surface wind speed, further hindering the PM2.5 dispersion, and consequently exacerbating the haze pollution in the NCP. Furthermore, when the near-surface PM2.5 mass concentration increases from around 50 to several hundred µg m−3, ARF contributes to the near-surface PM2.5 by more than 20 % during daytime in the NCP, substantially aggravating the heavy haze formation. However, when the near-surface PM2.5 concentration is less than around 50 µg m−3, ARF generally reduces the near-surface PM2.5 concentration due to the consequent perturbation of atmospheric dynamic fields.

scholarly journals Impact of the Green Light Program on haze pollution in the North China Plain, China

2019 ◽  
Author(s):  
Xin Long ◽  
Xuexi Tie ◽  
Jiamao Zhou ◽  
Wenting Dai ◽  
Xueke Li ◽  
...  
Keyword(s):  
Power Generation ◽  
Emission Reduction ◽  
North China Plain ◽  
North China ◽  
Thermal Power ◽  
Coal Consumption ◽  
The North ◽  
The North China Plain ◽  
Haze Pollution ◽  
Pm2.5 Concentration

Abstract. As the world's largest developing country, China undergoes the ever-increasing demand for electricity during the past few decades. In 1996, China launched the Green Lights Program (GLP), which becomes a national energy conservation activity for saving lighting electricity, as well as an effective reduction of the coal consumption for power generation. Despite of the great success of the GLP, its effects on haze pollution have not been investigated and well understood. This study focused to assess the potential coal-saving induced by the GLP and to estimate the consequent improvements of the haze pollutions in the North China Plain (NCP), because severe haze pollutions often occur in the NCP and a large amount of power plants locate in this region. The estimated potential coal-saving induced by the GLP can reach a massive value of 120–323 million tons, accounting for 6.7–18.0 % of the total coal consumption for thermal power generation in China. In December 2015, there was a massive potential emission reduction of air pollutants from thermal power generation in the NCP, which was estimated to be 20.0–53.8 Gg for NOx and 6.9–18.7 Gg for SO2. The potential emission reductions induced by the GLP played important roles in the haze formation, because the NOx and SO2 are important precursors for the formation of particles. To assess the impact of the GLP on haze pollution, sensitive studies were conducted by applying a regional chemical/dynamical model (WRF-CHEM). The model results suggest that in the lower limit case of emission reduction, the PM2.5 concentration decreases by 2–5 µg m−3 in large areas of the NCP. In the upper limit case of emission reduction, there was much more remarkable decrease in PM2.5 concentration (4–10 µg m−3). This study is a good example to illustrate that scientific innovation can induce important benefits on environment issues, such as haze pollution.

scholarly journals Is water vapor a key player of the wintertime haze in North China Plain?

2019 ◽  
Author(s):  
Jiarui Wu ◽  
Naifang Bei ◽  
Bo Hu ◽  
Suixin Liu ◽  
Meng Zhou ◽  
...  
Keyword(s):  
Water Vapor ◽  
North China Plain ◽  
North China ◽  
Temporal Variations ◽  
Effective Radius ◽  
Heterogeneous Reactions ◽  
Hygroscopic Growth ◽  
Near Surface ◽  
Haze Pollution ◽  
Average Contribution

Abstract. Water vapor has been proposed to amplify the severe haze pollution in China by enhancing the aerosol-radiation feedback (ARF). Observations have revealed that the near-surface PM2.5 concentrations ([PM2.5]) generally exhibits an increasing trend with relative humidity (RH) in North China Plain (NCP) during 2015 wintertime, indicating that the aerosol liquid water (ALW) caused by hygroscopic growth could play an important role in the PM2.5 formation and accumulation. Simulations during a persistent and heavy haze pollution episode from 05 December 2015 to 04 January 2016 in NCP were conducted using the WRF-CHEM model to comprehensively quantify contributions of the ALW effect to near-surface [PM2.5]. The WRF-CHEM model generally performs reasonably well in simulating the temporal variations of RH against measurements in NCP. The factor separation approach (FSA) was used to evaluate the contribution of the ALW effect on the ARF, photochemistry, and heterogeneous reactions to [PM2.5]. The ALW not only augments particle sizes to enhance aerosol backward scattering, but also increases the effective radius to favor aerosol forward scattering. The contribution of the ALW effect on the ARF and photochemistry to near [PM2.5] is not significant, generally within 1.0 μg m−3 on average in NCP during the episode. Serving as an excellent substrate for heterogeneous reactions, the ALW substantially enhances the secondary aerosol (SA) formation, with an average contribution of 71 %, 10 %, 26 %, and 48 % to near-surface sulfate, nitrate, ammonium, and secondary organic aerosol concentrations. Nevertheless, the SA enhancement due to the ALW decreases the aerosol optical depth and increases the effective radius to weaken the ARF, reducing near-surface primary aerosols. The contribution of the ALW total effect to near-surface [PM2.5] is 17.5 % on average, which is overwhelmingly dominated by enhanced SA. Model sensitivities also show that when the RH is less than 80 %, the ALW progressively increases near-surface [PM2.5], but commences to decrease when the RH exceeding 80% due to the high occurrence frequencies of precipitation.

scholarly journals Is water vapor a key player of the wintertime haze in North China Plain?

2019 ◽  
Vol 19 (13) ◽  
pp. 8721-8739 ◽  
Author(s):  
Jiarui Wu ◽  
Naifang Bei ◽  
Bo Hu ◽  
Suixin Liu ◽  
Meng Zhou ◽  
...  
Keyword(s):  
Water Vapor ◽  
North China Plain ◽  
North China ◽  
Temporal Variations ◽  
Effective Radius ◽  
Heterogeneous Reactions ◽  
Hygroscopic Growth ◽  
Near Surface ◽  
The North ◽  
Haze Pollution

Abstract. Water vapor has been proposed to amplify the severe haze pollution in China by enhancing the aerosol–radiation feedback (ARF). Observations have revealed that the near-surface PM2.5 concentrations ([PM2.5]) generally exhibit an increasing trend with relative humidity (RH) in the North China Plain (NCP) during 2015 wintertime, indicating that the aerosol liquid water (ALW) caused by hygroscopic growth could play an important role in the PM2.5 formation and accumulation. Simulations during a persistent and heavy haze pollution episode from 5 December 2015 to 4 January 2016 in the NCP were conducted using the WRF-Chem Model to comprehensively quantify contributions of the ALW effect to near-surface [PM2.5]. The WRF-Chem Model generally performs reasonably well in simulating the temporal variations in RH against measurements in the NCP. The factor separation approach (FSA) was used to evaluate the contribution of the ALW effect on the ARF, photochemistry, and heterogeneous reactions to [PM2.5]. The ALW not only augments particle sizes to enhance aerosol backward scattering but also increases the effective radius to favor aerosol forward scattering. The contribution of the ALW effect on the ARF and photochemistry to near-surface [PM2.5] is not significant, being generally within 1.0 µg m−3 on average in the NCP during the episode. Serving as an excellent substrate for heterogeneous reactions, the ALW substantially enhances the secondary aerosol (SA) formation, with an average contribution of 71 %, 10 %, 26 %, and 48 % to near-surface sulfate, nitrate, ammonium, and secondary organic aerosol concentrations. Nevertheless, the SA enhancement due to the ALW decreases the aerosol optical depth and increases the effective radius to weaken the ARF, reducing near-surface primary aerosols. The contribution of the ALW total effect to near-surface [PM2.5] is 17.5 % on average, which is overwhelmingly dominated by enhanced SA. Model sensitivities also show that when the RH is less than 80 %, the ALW progressively increases near-surface [PM2.5] but commences to decrease when the RH exceeds 80 % due to the high occurrence frequencies of precipitation.

scholarly journals Air Quality and Climate Change, Topic 3 of the Model Inter-Comparison Study for Asia Phase III (MICS-Asia III), Part I: overview and model evaluation

2017 ◽  
Author(s):  
Meng Gao ◽  
Zhiwei Han ◽  
Zirui Liu ◽  
Meng Li ◽  
Jinyuan Xin ◽  
...  
Keyword(s):  
Air Quality ◽  
Model Evaluation ◽  
Air Pollutants ◽  
North China ◽  
Correlation Coefficients ◽  
Phase Iii ◽  
Comparison Study ◽  
Model Ensemble ◽  
Near Surface ◽  
Ensemble Mean

Abstract. Topic 3 of the Model Inter-Comparison Study for Asia (MICS-Asia) Phase III examines how online coupled air quality models perform in simulating high aerosol pollution in the North China Plain region during wintertime haze events and evaluates the importance of aerosol radiative and microphysical feedbacks. A comprehensive overview of the MICS-ASIA III Topic 3 study design, including descriptions of participating models and model inputs, the experimental designs, and results of model evaluation, are presented. Two winter months (January 2010 and January 2013) were selected as study periods, when severe haze occurred in North China. Simulations were designed to evaluate radiative and microphysical feedbacks, together and separately, relative to simulations without feedbacks. Six modeling groups from China, Korea and the United States submitted results from seven applications of online coupled chemistry-meteorology models. Results are compared to meteorology and air quality measurements, including the Campaign on Atmospheric Aerosol Research Network of China (CARE-China) network, and the Acid Deposition Monitoring Network in East Asia (EANET). The analysis focuses on model evaluations and aerosol effects on meteorology and air quality, and potentially other interesting topics, such as the impacts of model resolutions on aerosol-radiation-weather interactions. The model evaluations for January 2010 show that current online-coupled meteorology-chemistry model can generally well reproduced meteorological features and variations of major air pollutants, including aerosol concentrations. The correlation coefficients between multi-model ensemble mean and observed near-surface temperature, water vapor mixing ratio and wind speeds can reach as high as 0.99, 0.99 and 0.98. The correlation coefficients between multi-model ensemble mean and the CARE-China observed near-surface air pollutants range from 0.51 to 0.94 (0.51 for ozone and 0.94 for PM2.5). However, large discrepancies exist between simulated aerosol chemical compositions from different models, which is due to different parameterizations of chemical reactions. The coefficient of variation (standard deviation divided by average) can reach above 1.3 for sulfate in Beijing, and above 1.6 for nitrate and organic aerosol in coastal regions, indicating these compositions are less consistent from different models. During clean periods, simulated Aerosol Optical Depths (AOD) from different models are consistent, but peak values differ during severe haze event, which can be explained by the differences in simulated inorganic aerosol concentrations and the hygroscopic growth efficiency (affected by varied RH). These results provide some brief senses of how current online-coupled meteorology-chemistry models reproduce severe haze events, and some directions for future model improvements.

scholarly journals Aerosol chemistry and particle growth events at an urban downwind site in North China Plain

2018 ◽  
Vol 18 (19) ◽  
pp. 14637-14651 ◽  
Author(s):  
Yingjie Zhang ◽  
Wei Du ◽  
Yuying Wang ◽  
Qingqing Wang ◽  
Haofei Wang ◽  
...  
Keyword(s):  
Growth Rates ◽  
North China Plain ◽  
North China ◽  
Particle Growth ◽  
Early Morning ◽  
Scanning Mobility Particle Sizer ◽  
Average Mass ◽  
The North ◽  
Haze Pollution ◽  
Engine Version

Abstract. The North China Plain (NCP) has experienced frequent severe haze pollution events in recent years. While extensive measurements have been made in megacities, aerosol sources, processes, and particle growth at urban downwind sites remain less understood. Here, an aerosol chemical speciation monitor and a scanning mobility particle sizer, along with a suite of collocated instruments, were deployed at the downwind site of Xingtai, a highly polluted city in the NCP, for real-time measurements of submicron aerosol (PM1) species and particle number size distributions during May and June 2016. The average mass concentration of PM1 was 30.5 (±19.4) µg m−3, which is significantly lower than that during wintertime. Organic aerosols (OAs) constituted the major fraction of PM1 (38 %), followed by sulfate (25 %) and nitrate (14 %). Positive matrix factorization with the multilinear engine version 2 showed that oxygenated OA (OOA) was the dominant species in OA throughout the study, on average accounting for 78 % of OA, while traffic and cooking emissions both accounted for 11 % of OA. Our results highlight that aerosol particles at the urban downwind site were highly aged and mainly from secondary formation. However, the diurnal cycle also illustrated the substantial influence of urban emissions on downwind sites, which are characterized by similar pronounced early morning peaks for most aerosol species. New particle formation and growth events were also frequently observed (58 % of the time) on both clean and polluted days. Particle growth rates varied from 1.2 to 4.9 nm h−1 and our results showed that sulfate and OOA played important roles in particle growth during clean periods, while OOA was more important than sulfate during polluted events. Further analyses showed that particle growth rates have no clear dependence on air mass trajectories.

Study on Regional Distribution of Air Pollutants in North China Plain by Mobile DOAS

2016 ◽  
Vol 36 (4) ◽  
pp. 0401001
Author(s):  
牟福生 Mou Fusheng ◽  
李昂 Li Ang ◽  
谢品华 Xie Pinhua ◽  
吴丰成 Wu Fengcheng ◽  
张杰 Zhang Jie ◽  
...  
Keyword(s):  
Air Pollutants ◽  
North China Plain ◽  
North China ◽  
Regional Distribution

scholarly journals Measuring the Vertical Profiles of Aerosol Extinction in the Lower Troposphere by MAX-DOAS at a Rural Site in the North China Plain

Atmosphere ◽  
2020 ◽  
Vol 11 (10) ◽  
pp. 1037
Author(s):  
Siyang Cheng ◽  
Junli Jin ◽  
Jianzhong Ma ◽  
Xiaobin Xu ◽  
Liang Ran ◽  
...  
Keyword(s):  
North China Plain ◽  
North China ◽  
Lower Troposphere ◽  
Temporal Variations ◽  
Rural Site ◽  
Optical Absorption Spectroscopy ◽  
Aerosol Extinction ◽  
Vertical Profiles ◽  
Near Surface ◽  
The North

Ground-based multi-axis differential optical absorption spectroscopy (MAX-DOAS) measurements were performed during the summer (13 June–20 August) of 2014 at a rural site in North China Plain. The vertical profiles of aerosol extinction (AE) in the lower troposphere were retrieved to analyze the temporal variations of AE profiles, near-surface AE, and aerosol optical depth (AOD). The average AOD and near-surface AE over the period of study were 0.51 ± 0.26 and 0.33 ± 0.18 km−1 during the effective observation period, respectively. High AE events and elevated AE layers were identified based on the time series of hourly AE profiles, near-surface AEs and AODs. It is found that in addition to the planetary boundary layer height (PBLH) and relative humidity (RH), the variations in the wind field have large impacts on the near-surface AE, AOD, and AE profile. Among 16 wind sectors, higher AOD or AE occur mostly in the directions of the cities upstream. The diurnal variations of the AE profiles, AODs and near-surface AEs are significant and influenced mainly by the source emissions, PBLH, and RH. The AE profile shape from MAX-DOAS measurement is generally in agreement with that from light detection and ranging (lidar) observations, although the AE absolute levels are different. Overall, ground-based MAX-DOAS can serve as a supplement to measure the AE vertical profiles in the lower troposphere.

Sign in / Sign up

Export Citation Format

Share Document