Experimental station for ultrafast extreme ultraviolet spectroscopy for non-equilibrium dynamics in warm dense matter

AbstractExperiments featuring non-equilibrium glassy dynamics under temperature changes still await interpretation. There is a widespread feeling that temperature chaos (an extreme sensitivity of the glass to temperature changes) should play a major role but, up to now, this phenomenon has been investigated solely under equilibrium conditions. In fact, the very existence of a chaotic effect in the non-equilibrium dynamics is yet to be established. In this article, we tackle this problem through a large simulation of the 3D Edwards-Anderson model, carried out on the Janus II supercomputer. We find a dynamic effect that closely parallels equilibrium temperature chaos. This dynamic temperature-chaos effect is spatially heterogeneous to a large degree and turns out to be controlled by the spin-glass coherence length ξ. Indeed, an emerging length-scale ξ* rules the crossover from weak (at ξ ≪ ξ*) to strong chaos (ξ ≫ ξ*). Extrapolations of ξ* to relevant experimental conditions are provided.

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Warm dense matter simulation via electron temperature dependent deep potential molecular dynamics

Physics of Plasmas ◽

10.1063/5.0023265 ◽

2020 ◽

Vol 27 (12) ◽

pp. 122704

Author(s):

Yuzhi Zhang ◽

Chang Gao ◽

Qianrui Liu ◽

Linfeng Zhang ◽

Han Wang ◽

...

Keyword(s):

Molecular Dynamics ◽

Electron Temperature ◽

Dense Matter ◽

Temperature Dependent ◽

Warm Dense Matter

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Epidemic growth and Griffiths effects on an emergent network of excited atoms

Nature Communications ◽

10.1038/s41467-020-20333-7 ◽

2021 ◽

Vol 12 (1) ◽

Author(s):

T. M. Wintermantel ◽

M. Buchhold ◽

S. Shevate ◽

M. Morgado ◽

Y. Wang ◽

...

Keyword(s):

Complex Systems ◽

Power Laws ◽

Excitation Density ◽

Griffiths Phase ◽

Many Body ◽

Excited Atoms ◽

Equilibrium Dynamics ◽

Many Body Systems ◽

Excitation Number ◽

Non Equilibrium

AbstractWhether it be physical, biological or social processes, complex systems exhibit dynamics that are exceedingly difficult to understand or predict from underlying principles. Here we report a striking correspondence between the excitation dynamics of a laser driven gas of Rydberg atoms and the spreading of diseases, which in turn opens up a controllable platform for studying non-equilibrium dynamics on complex networks. The competition between facilitated excitation and spontaneous decay results in sub-exponential growth of the excitation number, which is empirically observed in real epidemics. Based on this we develop a quantitative microscopic susceptible-infected-susceptible model which links the growth and final excitation density to the dynamics of an emergent heterogeneous network and rare active region effects associated to an extended Griffiths phase. This provides physical insights into the nature of non-equilibrium criticality in driven many-body systems and the mechanisms leading to non-universal power-laws in the dynamics of complex systems.

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An Investigation into the Approximations Used in Wave Packet Molecular Dynamics for the Study of Warm Dense Matter

Plasma ◽

10.3390/plasma4020020 ◽

2021 ◽

Vol 4 (2) ◽

pp. 294-308

Author(s):

William A. Angermeier ◽

Thomas G. White

Keyword(s):

Molecular Dynamics ◽

Wave Packet ◽

Hydrogen Plasma ◽

Valence Bond ◽

Dense Matter ◽

Basis Set ◽

Warm Dense Matter ◽

Scaling Parameters ◽

Oppenheimer Approximation ◽

Semi Empirical

Wave packet molecular dynamics (WPMD) has recently received a lot of attention as a computationally fast tool with which to study dynamical processes in warm dense matter beyond the Born–Oppenheimer approximation. These techniques, typically, employ many approximations to achieve computational efficiency while implementing semi-empirical scaling parameters to retain accuracy. We investigated three of the main approximations ubiquitous to WPMD: a restricted basis set, approximations to exchange, and the lack of correlation. We examined each of these approximations in regard to atomic and molecular hydrogen in addition to a dense hydrogen plasma. We found that the biggest improvement to WPMD comes from combining a two-Gaussian basis with a semi-empirical correction based on the valence-bond wave function. A single parameter scales this correction to match experimental pressures of dense hydrogen. Ultimately, we found that semi-empirical scaling parameters are necessary to correct for the main approximations in WPMD. However, reducing the scaling parameters for more ab-initio terms gives more accurate results and displays the underlying physics more readily.

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