Investigation of 6S 1/2–8S 1/2 two-photon transition of cesium atoms by a single 822 nm laser

We experimentally investigate the 6S 1/2–8S 1/2 two-photon transition in cesium vapor by a single laser. A blue (455.5 and 459.3 nm) fluorescence signal is observed as a result of 822.5 nm laser beams illuminating the Cs vapor with a counter-propagating configuration. The dependences of the fluorescence intensity on the polarization combinations of the laser beams, laser power and vapor temperature are studied to obtain optimal experimental parameters. The frequency difference between the two hyperfine components of 4158 (7) MHz is measured with a Fabry–Perot interferometer as a frequency reference. Such a large spectral isolation and the insensitivity to the Earth’s magnetic field enable the 6S 1/2–8S 1/2 transition to be a stable frequency standard candidate for a frequency-doubled 1644 nm laser in the U-band window for quantum telecommunication.