Long term operation of high concentration powdered activated carbon membrane bio-reactor for advanced water treatment

2004 ◽  
Vol 50 (8) ◽  
pp. 81-87 ◽  
Author(s):  
G.T. Seo ◽  
C.D. Moon ◽  
S.W. Chang ◽  
S.H. Lee
Keyword(s):  
Activated Carbon ◽  
Water Treatment ◽  
Membrane Bioreactor ◽  
Treatment Plant ◽  
Drinking Water Treatment ◽  
Powdered Activated Carbon ◽  
Carbon Membrane ◽  
High Concentration ◽  
Term Operation ◽  
Nakdong River Basin

A pilot scale experiment was conducted to evaluate the performance of a membrane bioreactor filled with high concentration powdered activated carbon. This hybrid system has great potential to substitute for existing GAC or O3/BAC processes in the drinking water treatment train. The system was installed at a water treatment plant located downstream of the Nakdong river basin, Korea. Effluent of rapid sand filter was used as influent of the system which consists of PAC bio-reactor, submerged MF membrane module and air supply facility. PAC concentration of 20 g/L was maintained at the beginning of the experiment and it was increased to 40 g/L. The PAC has not been changed during the operational periods. The membrane was a hollow fiber type with pore sizes of 0.1 and 0.4 µm. It was apparent that the high PAC concentration could prevent membrane fouling. 40 g/L PAC was more effective to reduce the filtration resistance than 20 g/L. At the flux of 0.36 m/d, TMP was maintained less than 40 kPa for about 3 months by intermittent suction type operation (12 min suction/3 min idling). Adsorption was the dominant role to remove DOC at the initial operational period. However the biological effect was gradually increased after around 3 months operation. Constant DOC removal could be maintained at about 40% without any trouble and then a tremendous reduction of DBPs (HAA5 and THM) higher than 85% was achieved. Full nitrification was observed at the controlled influent ammonia nitrogen concentration of 3 and 7 mg/L. pH was an important parameter to keep stable ammonia oxidation. From almost two years of operation, it is clear that the PAC membrane bioreactor is highly applicable for advanced water treatment under the recent situation of more stringent DBPs regulation in Korea.

scholarly journals Removal of radio N-nitrosodimethylamine (NDMA) from drinking water by coagulation and Powdered Activated Carbon (PAC) adsorption

2009 ◽  
Vol 2 (1) ◽  
pp. 79-100 ◽  
Author(s):  
J. Chung ◽  
Y. Yoon ◽  
M. Kim ◽  
S.-B. Lee ◽  
H.-J. Kim ◽  
...  
Keyword(s):  
Drinking Water ◽  
Activated Carbon ◽  
Water Treatment ◽  
Background Electrolyte ◽  
Treatment Plant ◽  
Drinking Water Treatment ◽  
Powdered Activated Carbon ◽  
Individual Treatment ◽  
Solution Ph ◽  
Treatment Processes

Abstract. The presence of N-nitrosodimethylamine (NDMA) in drinking water supplies has raised concern over its removal by common drinking water treatment processes. A simple detection method based on scintillation spectroscopy has been used to quantify the concentration of 14C-labeled NDMA at various ratios of sample to scintillation liquid. Without sample pretreatment, the method detection limits are 0.91, 0.98, 1.23, and 1.45 ng/L of NDMA at scintillation intensity ratios of 10:10, 5:15, 15:5, and 2.5:17.5 (sample: scintillation liquid), respectively. The scintillation intensity in all cases is linear (R2>0.99) and is in the range of 0 to 100 ng/L of NDMA. In addition, because scintillation intensity is independent of solution pH, conductivity, and background electrolyte ion types, a separate calibration curve is unnecessary for NDMA samples at different solution conditions. Bench-scale experiments were performed to simulate individual treatment processes, which include coagulation and adsorption by powdered activated carbon (PAC), as used in a drinking water treatment plant, and biosorption, a technique used in biological treatment of waste water. The commonly used coagulation process for particulate control and biosorption is ineffective for removing NDMA (<10% by coagulation and <20% by biosorption). However, high doses of PAC may be applied to remove NDMA.

Ammonia oxidation at low temperature in a high concentration powdered activated carbon membrane bioreactor

2002 ◽  
Vol 2 (2) ◽  
pp. 169-176 ◽  
Author(s):  
G. Seo ◽  
S. Takizawa ◽  
S. Ohgaki
Keyword(s):  
Activated Carbon ◽  
Water Temperature ◽  
Membrane Bioreactor ◽  
Ammonia Oxidation ◽  
Hollow Fiber Membrane ◽  
Powdered Activated Carbon ◽  
Carbon Membrane ◽  
High Concentration ◽  
Filtration Resistance ◽  
Cake Layer

In this study, a membrane bioreactor (MBR) with high concentration of powdered activated carbon was investigated to enhance the oxidation of ammonia at a water temperature lower than 4°C. A semi-pilot scale submersed suction type MBR was operated with a hollow fiber membrane module having a nominal pore size of 0.1μm and an effective filtration area of 0.05 m2. A powder activated carbon (PAC) concentration of 40 g/L was maintained in the reactor and the PAC was not replaced during the experiment. A control reactor without PAC was also operated for comparison. Water temperature of both reactors was controlled at 25, 10, 4 and 2°C. At a water temperature of 4°C, the influent ammonia nitrogen of 10 mg/L was removed completely in the reactor with PAC. On the other hand, the effluent concentration of the control reactor was fluctuated in a range of 3-6 mg/L. In addition, nitrite nitrogen was detected in the control reactor up to a maximum concentration of 6 mg/L at the same temperature. Still high removal efficiency was obtained in the reactor with PAC even at 2°C, but almost no ammonia oxidation was observed in the control reactor. The average ammonia oxidation rate of the powdered activated carbon reactor was 1.3-3.2 mg/L.h, which is 4.5 times higher than that of the control (0.51-0.63 mg/L.h). Filtration resistance was 2.45 × 1012m-1 for the reactor with PAC, which is one order lower than that of the control reactor (1.64 × 1013m-1). The microbial cake layer on the membrane surface caused the larger filtration resistance for the control reactor. Only one chemical cleaning was conducted for the membrane in the PAC reactor at the flux of 0.4-0.7 m/d while 3 times cleaning was required for that of the control.

A pilot-scale study of a powdered activated carbon-membrane bioreactor for the treatment of water with a high concentration of ammonia

2016 ◽  
Vol 2 (1) ◽  
pp. 125-133 ◽  
Author(s):  
Senlin Shao ◽  
Fangshu Qu ◽  
Heng Liang ◽  
Haiqing Chang ◽  
Huarong Yu ◽  
...  
Keyword(s):  
Activated Carbon ◽  
Membrane Bioreactor ◽  
Pilot Scale ◽  
Ammonia Removal ◽  
Powdered Activated Carbon ◽  
Carbon Membrane ◽  
High Concentration

Ammonia removal was highly impacted by temperature and alkalinity. Fouling cake could remove a certain amount of ammonia.

scholarly journals Removal of radio N-nitrosodimethylamine (NDMA) from drinking water by coagulation and Powdered Activated Carbon (PAC) adsorption

2009 ◽  
Vol 2 (2) ◽  
pp. 49-55 ◽  
Author(s):  
J. Chung ◽  
Y. Yoon ◽  
M. Kim ◽  
S.-B. Lee ◽  
H.-J. Kim ◽  
...  
Keyword(s):  
Drinking Water ◽  
Activated Carbon ◽  
Water Treatment ◽  
Background Electrolyte ◽  
Treatment Plant ◽  
Drinking Water Treatment ◽  
Powdered Activated Carbon ◽  
Individual Treatment ◽  
Solution Ph ◽  
Treatment Processes

Abstract. The presence of N-nitrosodimethylamine (NDMA) in drinking water supplies has raised concern over its removal by common drinking water treatment processes. However, only limited studies have been examined to evaluate the potential removal of NDMA by numerous water treatment technologies within a realistic range (i.e., sub μg/L) of NDMA levels in natural water due to analytical availability. In this study, a simple detection method based on scintillation spectroscopy has been used to quantify the concentration of 14C-labeled NDMA at various ratios of sample to scintillation liquid. Without sample pretreatment, the method detection limits are 0.91, 0.98, 1.23, and 1.45 ng/L of NDMA at scintillation intensity ratios of 10:10, 5:15, 15:5, and 2.5:17.5 (sample: scintillation liquid), respectively. The scintillation intensity in all cases is linear (R2>0.99) and is in the range of 0 to 100 ng/L of NDMA. In addition, because scintillation intensity is independent of solution pH, conductivity, and background electrolyte ion types, a separate calibration curve is unnecessary for NDMA samples at different solution conditions. Bench-scale experiments were performed to simulate individual treatment processes, which include coagulation and adsorption by powdered activated carbon (PAC), as used in a drinking water treatment plant, and biosorption, a technique used in biological treatment of waste water. The results show that coagulation and biosorption may not be appropriate mechanisms to remove NDMA (i.e., hydrophilic based on its low octanol-water partitioning coefficient, Log Kow=0.57). However, relatively high removal of NDMA (approximately 50%) was obtained by PAC at high PAC dosages and longer contact times.

scholarly journals Pesticide removals in the nitrifying expanded-bed filter at drinking water treatment plant

2020 ◽  
Vol 15 (1) ◽  
pp. 1-13
Author(s):  
Nguyet Thi-Minh Dao ◽  
The-Anh Nguyen ◽  
Viet-Anh Nguyen ◽  
Mitsuharu Terashima ◽  
Hidenari Yasui
Keyword(s):  
Drinking Water ◽  
Activated Carbon ◽  
Water Treatment ◽  
Treatment Plant ◽  
Drinking Water Treatment ◽  
Cost Effective ◽  
Water Treatment Plant ◽  
Field Analysis ◽  
Expanded Bed ◽  
Biological Activated Carbon

The occurrence of pesticides even at low concentrations in drinking water sources might induce potential risks to public health. This study aimed to investigate the removal mechanisms of eight pesticides by the nitrifying expanded-bed filter using biological activated carbon media at the pretreatment of a drinking water plant. The field analysis demonstrated that four pesticides Flutolanil, Buprofezin, Chlorpyrifos, and Fenobucard, were removed at 82%, 55%, 54%, and 52% respectively, while others were not significantly removed. Under controlled laboratory conditions with continuous and batch experiments, the adsorption onto the biological activated carbon media was demonstrated to be the main removal pathway of the pesticides. The contribution of microorganisms to the pesticide removals was rather limited. The pesticide removals observed in the field reactor was speculated to be the adsorption on the suspended solids presented in the influent water. The obtained results highlighted the need to apply a more efficient and cost-effective technology to remove the pesticide in the drinking water treatment process. Keywords: biological activated carbon; drinking water treatment; nitrifying expanded-bed filter; pesticide removal.

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