scholarly journals The impact of residential combustion emissions on atmospheric aerosol, human health, and climate

2016 ◽  
Vol 16 (2) ◽  
pp. 873-905 ◽  
Author(s):  
E. W. Butt ◽  
A. Rap ◽  
A. Schmidt ◽  
C. E. Scott ◽  
K. J. Pringle ◽  
...  
Keyword(s):  
Eastern Europe ◽  
Human Health ◽  
Atmospheric Aerosol ◽  
Radiative Transfer Model ◽  
Transfer Model ◽  
So2 Emissions ◽  
Residential Sector ◽  
Residential Combustion ◽  
Combustion Emissions ◽  
The Impact

Abstract. Combustion of fuels in the residential sector for cooking and heating results in the emission of aerosol and aerosol precursors impacting air quality, human health, and climate. Residential emissions are dominated by the combustion of solid fuels. We use a global aerosol microphysics model to simulate the impact of residential fuel combustion on atmospheric aerosol for the year 2000. The model underestimates black carbon (BC) and organic carbon (OC) mass concentrations observed over Asia, Eastern Europe, and Africa, with better prediction when carbonaceous emissions from the residential sector are doubled. Observed seasonal variability of BC and OC concentrations are better simulated when residential emissions include a seasonal cycle. The largest contributions of residential emissions to annual surface mean particulate matter (PM2.5) concentrations are simulated for East Asia, South Asia, and Eastern Europe. We use a concentration response function to estimate the human health impact due to long-term exposure to ambient PM2.5 from residential emissions. We estimate global annual excess adult (>  30 years of age) premature mortality (due to both cardiopulmonary disease and lung cancer) to be 308 000 (113 300–497 000, 5th to 95th percentile uncertainty range) for monthly varying residential emissions and 517 000 (192 000–827 000) when residential carbonaceous emissions are doubled. Mortality due to residential emissions is greatest in Asia, with China and India accounting for 50 % of simulated global excess mortality. Using an offline radiative transfer model we estimate that residential emissions exert a global annual mean direct radiative effect between −66 and +21 mW m−2, with sensitivity to the residential emission flux and the assumed ratio of BC, OC, and SO2 emissions. Residential emissions exert a global annual mean first aerosol indirect effect of between −52 and −16 mW m−2, which is sensitive to the assumed size distribution of carbonaceous emissions. Overall, our results demonstrate that reducing residential combustion emissions would have substantial benefits for human health through reductions in ambient PM2.5 concentrations.

scholarly journals The impact of residential combustion emissions on atmospheric aerosol, human health and climate

2015 ◽  
Vol 15 (14) ◽  
pp. 20449-20520 ◽  
Author(s):  
E. W. Butt ◽  
A. Rap ◽  
A. Schmidt ◽  
C. E. Scott ◽  
K. J. Pringle ◽  
...  
Keyword(s):  
Eastern Europe ◽  
Human Health ◽  
Atmospheric Aerosol ◽  
Radiative Transfer Model ◽  
Transfer Model ◽  
So2 Emissions ◽  
Residential Sector ◽  
Residential Combustion ◽  
Combustion Emissions ◽  
The Impact

Abstract. Combustion of fuels in the residential sector for cooking and heating, results in the emission of aerosol and aerosol precursors impacting air quality, human health and climate. Residential emissions are dominated by the combustion of solid fuels. We use a global aerosol microphysics model to simulate the uncertainties in the impact of residential fuel combustion on atmospheric aerosol. The model underestimates black carbon (BC) and organic carbon (OC) mass concentrations observed over Asia, Eastern Europe and Africa, with better prediction when carbonaceous emissions from the residential sector are doubled. Observed seasonal variability of BC and OC concentrations are better simulated when residential emissions include a seasonal cycle. The largest contributions of residential emissions to annual surface mean particulate matter (PM2.5) concentrations are simulated for East Asia, South Asia and Eastern Europe. We use a concentration response function to estimate the health impact due to long-term exposure to ambient PM2.5 from residential emissions. We estimate global annual excess adult (> 30 years of age) premature mortality of 308 000 (113 300–497 000, 5th to 95th percentile uncertainty range) for monthly varying residential emissions and 517 000 (192 000–827 000) when residential carbonaceous emissions are doubled. Mortality due to residential emissions is greatest in Asia, with China and India accounting for 50 % of simulated global excess mortality. Using an offline radiative transfer model we estimate that residential emissions exert a global annual mean direct radiative effect of between −66 and +21 mW m-2, with sensitivity to the residential emission flux and the assumed ratio of BC, OC and SO2 emissions. Residential emissions exert a global annual mean first aerosol indirect effect of between −52 and −16 mW m-2, which is sensitive to the assumed size distribution of carbonaceous emissions. Overall, our results demonstrate that reducing residential combustion emissions would have substantial benefits for human health through reductions in ambient PM2.5 concentrations.

scholarly journals Analysis of actinic flux profiles measured from an ozonesonde balloon

2015 ◽  
Vol 15 (8) ◽  
pp. 4131-4144 ◽  
Author(s):  
P. Wang ◽  
M. Allaart ◽  
W. H. Knap ◽  
P. Stammes
Keyword(s):  
Atmospheric Chemistry ◽  
Low Cost ◽  
Green Light ◽  
Single Layer ◽  
Radiative Transfer Model ◽  
Cloud Base ◽  
Transfer Model ◽  
Actinic Flux ◽  
Clear Sky ◽  
The Impact

Abstract. A green light sensor has been developed at KNMI to measure actinic flux profiles using an ozonesonde balloon. In total, 63 launches with ascending and descending profiles were performed between 2006 and 2010. The measured uncalibrated actinic flux profiles are analysed using the Doubling–Adding KNMI (DAK) radiative transfer model. Values of the cloud optical thickness (COT) along the flight track were taken from the Spinning Enhanced Visible and Infrared Imager (SEVIRI) Cloud Physical Properties (CPP) product. The impact of clouds on the actinic flux profile is evaluated on the basis of the cloud modification factor (CMF) at the cloud top and cloud base, which is the ratio between the actinic fluxes for cloudy and clear-sky scenes. The impact of clouds on the actinic flux is clearly detected: the largest enhancement occurs at the cloud top due to multiple scattering. The actinic flux decreases almost linearly from cloud top to cloud base. Above the cloud top the actinic flux also increases compared to clear-sky scenes. We find that clouds can increase the actinic flux to 2.3 times the clear-sky value at cloud top and decrease it to about 0.05 at cloud base. The relationship between CMF and COT agrees well with DAK simulations, except for a few outliers. Good agreement is found between the DAK-simulated actinic flux profiles and the observations for single-layer clouds in fully overcast scenes. The instrument is suitable for operational balloon measurements because of its simplicity and low cost. It is worth further developing the instrument and launching it together with atmospheric chemistry composition sensors.

scholarly journals Data-Driven Localization Mappings in Filtering the Monsoon–Hadley Multicloud Convective Flows

2018 ◽  
Vol 146 (4) ◽  
pp. 1197-1218
Author(s):  
Michèle De La Chevrotière ◽  
John Harlim
Keyword(s):  
Learning Algorithm ◽  
Data Driven ◽  
Radiative Transfer Model ◽  
Transfer Model ◽  
Model Errors ◽  
Accurate Analysis ◽  
Perfect Model ◽  
Nonlinear Stochastic Model ◽  
Correlation Statistics ◽  
The Impact

This paper demonstrates the efficacy of data-driven localization mappings for assimilating satellite-like observations in a dynamical system of intermediate complexity. In particular, a sparse network of synthetic brightness temperature measurements is simulated using an idealized radiative transfer model and assimilated to the monsoon–Hadley multicloud model, a nonlinear stochastic model containing several thousands of model coordinates. A serial ensemble Kalman filter is implemented in which the empirical correlation statistics are improved using localization maps obtained from a supervised learning algorithm. The impact of the localization mappings is assessed in perfect-model observing system simulation experiments (OSSEs) as well as in the presence of model errors resulting from the misspecification of key convective closure parameters. In perfect-model OSSEs, the localization mappings that use adjacent correlations to improve the correlation estimated from small ensemble sizes produce robust accurate analysis estimates. In the presence of model error, the filter skills of the localization maps trained on perfect- and imperfect-model data are comparable.

The impact of time-dependent stellar activity on the atmospheric chemistry and observability of exoplanets

2021 ◽  
Author(s):  
Amy Louca ◽  
Yamila Miguel ◽  
Shang-Min Tsai
Keyword(s):  
Atmospheric Chemistry ◽  
Emission Spectra ◽  
Time Dependent ◽  
Radiative Transfer Model ◽  
Transfer Model ◽  
Stellar Spectrum ◽  
Stellar Spectra ◽  
Chemical Tracers ◽  
Atmospheric Escape ◽  
The Impact

<p class="p1">Observations of exoplanets used to characterize the chemistry and dynamics of atmospheres have developed considerably throughout the years. Nonetheless, it remains a difficult task to give a full and detailed description using solely observations. With future space missions such as JWST and ARIEL, both expected to be launched within this decade, it becomes even more crucial to be able to fully explain and predict the underlying chemistry and physics involved. In this research, we focus on modeling star-planet interactions by using synthetic flare spectra to predict chemical tracers for future missions. We make use of a chemical kinetics code that includes synthetic time-dependent stellar spectra and thermal atmospheric escape to simulate the atmospheres of known exoplanets. Using a radiative transfer model we then retrieve emission spectra. This ongoing study is focused on various known planetary systems of which the stellar spectrum has been obtained by the (mega-)MUSCLES collaboration. Preliminary results on these systems show that stellar flares and thermal escape can have a significant effect on the chemistry in atmospheres. </p>

scholarly journals Characterization of aerosol hygroscopicity using Raman lidar measurements at the EARLINET station of Payerne

2019 ◽  
Vol 19 (18) ◽  
pp. 11651-11668 ◽  
Author(s):  
Francisco Navas-Guzmán ◽  
Giovanni Martucci ◽  
Martine Collaud Coen ◽  
María José Granados-Muñoz ◽  
Maxime Hervo ◽  
...  
Keyword(s):  
Lower Troposphere ◽  
Radiative Transfer Model ◽  
Transfer Model ◽  
Raman Lidar ◽  
Hygroscopic Growth ◽  
Backscatter Coefficient ◽  
Radiative Balance ◽  
First Case ◽  
The Impact ◽  
Aerosol Hygroscopicity

Abstract. This study focuses on the analysis of aerosol hygroscopicity using remote sensing techniques. Continuous observations of aerosol backscatter coefficient (βaer), temperature (T) and water vapor mixing ratio (r) have been performed by means of a Raman lidar system at the aerological station of MeteoSwiss at Payerne (Switzerland) since 2008. These measurements allow us to monitor in a continuous way any change in aerosol properties as a function of the relative humidity (RH). These changes can be observed either in time at a constant altitude or in altitude at a constant time. The accuracy and precision of RH measurements from the lidar have been evaluated using the radiosonde (RS) technique as a reference. A total of 172 RS profiles were used in this intercomparison, which revealed a bias smaller than 4 % RH and a standard deviation smaller than 10 % RH between both techniques in the whole (in lower) troposphere at nighttime (at daytime), indicating the good performance of the lidar for characterizing RH. A methodology to identify situations favorable to studying aerosol hygroscopicity has been established, and the aerosol hygroscopicity has been characterized by means of the backscatter enhancement factor (fβ). Two case studies, corresponding to different types of aerosol, are used to illustrate the potential of this methodology. The first case corresponds to a mixture of rural aerosol and smoke particles (smoke mixture), which showed a higher hygroscopicity (fβ355=2.8 and fβ1064=1.8 in the RH range 73 %–97 %) than the second case, in which mineral dust was present (fβ355=1.2 and fβ1064=1.1 in the RH range 68 %–84 %). The higher sensitivity of the shortest wavelength to hygroscopic growth was qualitatively reproduced using Mie simulations. In addition, a good agreement was found between the hygroscopic analysis done in the vertical and in time for Case I, where the latter also allowed us to observe the hydration and dehydration of the smoke mixture. Finally, the impact of aerosol hygroscopicity on the Earth's radiative balance has been evaluated using the GAME (Global Atmospheric Model) radiative transfer model. The model showed an impact with an increase in absolute value of 2.4 W m−2 at the surface with respect to the dry conditions for the hygroscopic layer of Case I (smoke mixture).

scholarly journals Cloud sensitivity studies for stratospheric and lower mesospheric ozone profile retrievals from measurements of limb-scattered solar radiation

2009 ◽  
Vol 2 (2) ◽  
pp. 653-678 ◽  
Author(s):  
T. Sonkaew ◽  
V. V. Rozanov ◽  
C. von Savigny ◽  
A. Rozanov ◽  
H. Bovensmann ◽  
...  
Keyword(s):  
Solar Radiation ◽  
Relative Error ◽  
Optical Thickness ◽  
Radiative Transfer Model ◽  
Transfer Model ◽  
Absorption Bands ◽  
Ozone Profile ◽  
Mesospheric Ozone ◽  
Cloud Optical Thickness ◽  
The Impact

Abstract. Clouds in the atmosphere play an important role in reflection, absorption and transmission of solar radiation and thus affect trace gas retrievals. The main goal of this paper is to examine the sensitivity of stratospheric and lower mesospheric ozone retrievals from limb-scattered radiance measurements to clouds using the SCIATRAN radiative transfer model and retrieval package. The retrieval approach employed is optimal estimation, and the considered clouds are vertically and horizontally homogeneous. Assuming an aerosol-free atmosphere and Mie phase functions for cloud particles, we compute the relative error of ozone profile retrievals in a cloudy atmosphere if clouds are neglected in the retrieval. To access altitudes from the lower stratosphere up to the lower mesosphere, we combine the retrievals in the Chappuis and Hartley ozone absorption bands. We find significant cloud sensitivity of the limb ozone retrievals in the Chappuis bands at lower stratospheric altitudes. The relative error in the retrieved ozone concentrations gradually decreases with increasing altitude and becomes negligible above approximately 40 km. The parameters with the largest impact on the ozone retrievals are cloud optical thickness, ground albedo and solar zenith angle. Clouds with different geometrical thicknesses or different cloud altitudes have a similar impact on the ozone retrievals for a given cloud optical thickness value, if the clouds are outside the field of view of the instrument. The effective radius of water droplets has a small influence on the error, i.e., less than 0.5% at altitudes above the cloud top height. Furthermore, the impact of clouds on the ozone profile retrievals was found to have a rather small dependence on the solar azimuth angle (less than 1% for all possible azimuth angles). For the most frequent cloud types, the total error is below 6% above 15 km altitude, if clouds are completely neglected in the retrieval. Neglecting clouds in the ozone profile retrievals generally leads to a low bias for a low ground albedo and to a high bias for a high ground albedo, assuming that the ground albedo is well known.

scholarly journals Further evidence of important environmental information content in red-to-green ratios as depicted in paintings by great masters

2014 ◽  
Vol 14 (6) ◽  
pp. 2987-3015 ◽  
Author(s):  
C. S. Zerefos ◽  
P. Tetsis ◽  
A. Kazantzidis ◽  
V. Amiridis ◽  
S. C. Zerefos ◽  
...  
Keyword(s):  
Industrial Revolution ◽  
Ice Core ◽  
Volcanic Eruptions ◽  
Radiative Transfer Model ◽  
Independent Experiment ◽  
Accurate Information ◽  
Transfer Model ◽  
Optical Extinction ◽  
The Difference ◽  
The Impact

Abstract. We examine sunsets painted by famous artists as proxy information for the aerosol optical depth after major volcanic eruptions. Images derived from precision colour protocols applied to the paintings were compared to online images, and found that the latter, previously analysed, provide accurate information. Aerosol optical depths (AODs) at 550 nm, corresponding to Northern Hemisphere middle latitudes, calculated by introducing red-to-green (R / G) ratios from a large number of paintings to a radiative transfer model, were significantly correlated with independent proxies from stratospheric AOD and optical extinction data, the dust veil index, and ice core volcanic indices. AODs calculated from paintings were grouped into 50-year intervals from 1500 to 2000. The year of each eruption and the 3 following years were defined as "volcanic". The remaining "non-volcanic" years were used to provide additional evidence of a multidecadal increase in the atmospheric optical depths during the industrial "revolution". The increase of AOD at 550 nm calculated from the paintings grows from 0.15 in the middle 19th century to about 0.20 by the end of the 20th century. To corroborate our findings, an experiment was designed in which a master painter/colourist painted successive sunsets during and after the passage of Saharan aerosols over the island of Hydra in Greece. Independent solar radiometric measurements confirmed that the master colourist's R / G ratios which were used to model his AODs, matched the AOD values measured in situ by co-located sun photometers during the declining phase of the Saharan aerosol. An independent experiment was performed to understand the difference between R / G ratios calculated from a typical volcanic aerosol and those measured from the mineral aerosol during the Hydra experiment. It was found that the differences in terms of R / G ratios were small, ranging between −2.6% and +1.6%. Also, when analysing different parts of cloudless skies of paintings following major volcanic eruptions, any structural differences seen in the paintings had not altered the results discussed above. However, a detailed study on all possible sources of uncertainties involved (such as the impact of clouds on R / G ratios) still needs to be studied. Because of the large number of paintings studied, we tentatively propose the conclusion that regardless of the school, red-to-green ratios from great masters can provide independent proxy AODs that correlate with widely accepted proxies and with independent measurements.

Modelling understory light availability in a heterogeneous landscape using drone-derived structural parameters and a 3D radiative transfer model

2020 ◽  
Author(s):  
Dominic Fawcett ◽  
Jonathan Bennie ◽  
Karen Anderson
Keyword(s):  
Radiative Transfer ◽  
Vegetation Index ◽  
Structural Parameters ◽  
Point Clouds ◽  
Radiative Transfer Model ◽  
Transfer Model ◽  
Area Index ◽  
Vegetation Height ◽  
Plant Area Index ◽  
The Impact

<p>The light environment within vegetated landscapes is a key driver of microclimate, creating varied habitats over small spatial extents and controls the distribution of understory plant species. Modelling spatial variations of light at these scales requires finely resolved (< 1 m) information on topography and canopy properties. We demonstrate an approach to modelling spatial distributions and temporal progression of understory photosynthetically active radiation (PAR) utilising a three dimensional radiative transfer model (discrete anisotropic radiative transfer model: DART) where the scene is parameterised by drone-based data.</p><p>The study site, located in west Cornwall, UK, includes a small mixed woodland as well as isolated free-standing trees. Data were acquired from March to August 2019. Vegetation height and distribution were derived from point clouds generated from drone image data using structure-from-motion (SfM) photogrammetry. These data were supplemented by multi-temporal multispectral imagery (Parrot Sequoia camera) which were used to generate an empirical model by relating a vegetation index to plant area index derived from hemispherical photography taken over the same time period. Simulations of the 3D radiative budget were performed for the PAR wavelength interval (400 – 700 nm) using DART.</p><p>Besides maps of instantaneous above and below canopy irradiance, we provide models of daily light integrals (DLI) which are assessed against field validation measurements with PAR quantum sensors. We find relatively good agreement for simulated PAR in the woodland. The impact of simplifying assumptions regarding leaf angular distributions and optical properties are discussed. Finally, further opportunities which fine-grained drone data can provide in a radiative transfer context are highlighted.</p>

Impact of 3D cloud structures on tropospheric NO2 column measurements from UV-VIS sounders

2020 ◽  
Author(s):  
Huan Yu ◽  
Arve Kylling ◽  
Claudia Emde ◽  
Bernhard Mayer ◽  
Kerstin Stebel ◽  
...  
Keyword(s):  
Radiative Transfer ◽  
Mitigation Strategies ◽  
Trace Gas ◽  
Radiative Transfer Model ◽  
Transfer Model ◽  
Vertical Column ◽  
Ice Clouds ◽  
Cloud Data ◽  
One Step ◽  
The Impact

<p>Operational retrievals of tropospheric trace gases from space-borne spectrometers are made using 1D radiative transfer models. To minimize cloud effects generally only partially cloudy pixels are analysed using simplified cloud contamination treatments based on radiometric cloud fraction estimates and photon path length corrections based on oxygen collision pair (O<sub>2</sub>-O<sub>2</sub>) or O<sub>2</sub>A-absorption band measurements. In reality, however, the impact of clouds can be much more complex, involving scattering of clouds in neighbouring pixels and cloud shadow effects. Therefore, to go one step further, other correction methods may be envisaged that use sub-pixel cloud information from co-located imagers. Such methods require an understanding of the impact of clouds on the real 3D radiative transfer. We quantify this impact using the MYSTIC 3D radiative transfer model. The generation of realistic 3D input cloud fields, needed by MYSTIC (or any other 3D radiative transfer model), is non-trivial. We use cloud data generated by the ICOsahedral Non-hydrostatic (ICON) atmosphere model for a region including Germany, the Netherlands and parts of other surrounding countries. The model simulates realistic liquid and ice clouds with a horizontal spatial resolution of 156 m and it has been validated against ground-based and satellite-based observational data.</p><p>As a trace gas example, we study NO<sub>2</sub>, a key tropospheric trace gas measured by the atmospheric Sentinels. The MYSTIC 3D model simulates visible spectra, which are ingested in standard DOAS retrieval algorithms to retrieve the NO<sub>2</sub> column amount. Spectra are simulated for a number of realistic cloud scenarios, snow free surface albedos, and solar and satellite geometries typical of low-earth and geostationary orbits. The retrieved NO<sub>2</sub> vertical column densities (VCD) are compared with the true values to identify conditions where 3D cloud effects lead to significant biases on the NO<sub>2</sub> VCDs. A variety of possible mitigation strategies for such pixels are then explored.</p>

Sign in / Sign up

Export Citation Format

Share Document