scholarly journals Diurnal evolution of negative atmospheric ions above the boreal forest: From ground level to the free troposphere

2021 ◽  
Author(s):  
Lisa J. Beck ◽  
Siegfried Schobesberger ◽  
Heikki Junninen ◽  
Janne Lampilahti ◽  
Antti Manninen ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Boreal Forest ◽  
Diurnal Variation ◽  
Stable Boundary Layer ◽  
Mixing Layer ◽  
Particle Formation ◽  
Residual Layer ◽  
Free Troposphere ◽  
Ion Composition ◽  
Stable Boundary

Abstract. At SMEAR II research station in Hyytiälä, located in the Finnish boreal forest, the process of new particle formation and the role of ions has been investigated for almost 20 years near the ground and at canopy level. However, above SMEAR II, the vertical distribution and diurnal variation of these different atmospheric ions are poorly characterized. In this study, we assess the atmospheric ion composition in the stable boundary layer, residual layer, mixing layer and free troposphere, and the 5 evolution of these atmospheric ions due to photochemistry and turbulent mixing through the day. To measure the vertical profile of atmospheric ions, we developed a tailored setup for online mass spectrometric measurements, capable of being deployed in a Cessna 172 with minimal modifications. Simultaneously, instruments dedicated to aerosol properties measured in a second Cessna. We conducted a total of 16 measurement flights in May 2017, during the spring, which is the most active new particle formation season. A flight day typically consisted of three distinct flights through the day (dawn, morning and afternoon) to 10 observe the diurnal variation and at different altitudes (from 100 m to 3200 m above ground), and to capture the boundary layer development from stable boundary layer, residual layer to mixing layer, and the free troposphere. Our observations showed that the ion composition is distinctly different in each layer and depends on the air mass origin and time of the day. Before sunrise, the layers are separated from each other and have their own ion chemistry. We observed that the ions present within the stable layer are of the same composition as the ions measured at the canopy level. During daytime when the mixing layer evolved and the compounds are vertically mixed, we observed that highly oxidised organic molecules are distributed to the top of the boundary layer. The ion composition in the residual layer varies with each day, showing similarities with either the stable boundary layer or the free troposphere. Finally, within the free troposphere, we detected a variety of carboxylic acids and ions that are likely containing halogens, originating from the Arctic Sea.

scholarly journals Aerosol particle formation in the upper residual layer

2021 ◽  
Vol 21 (10) ◽  
pp. 7901-7915
Author(s):  
Janne Lampilahti ◽  
Katri Leino ◽  
Antti Manninen ◽  
Pyry Poutanen ◽  
Anna Franck ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Boreal Forest ◽  
Mixed Layer ◽  
Cloud Condensation Nuclei ◽  
Large Fraction ◽  
Aerosol Particles ◽  
Lower Troposphere ◽  
Particle Formation ◽  
Residual Layer ◽  
Forest Environment

Abstract. According to current estimates, atmospheric new particle formation (NPF) produces a large fraction of aerosol particles and cloud condensation nuclei in the Earth's atmosphere, which have implications for health and climate. Despite recent advances, atmospheric NPF is still insufficiently understood in the lower troposphere, especially above the mixed layer (ML). This paper presents new results from co-located airborne and ground-based measurements in a boreal forest environment, showing that many NPF events (∼42 %) appear to start in the topmost part of the residual layer (RL). The freshly formed particles may be entrained into the growing mixed layer (ML) where they continue to grow in size, similar to the aerosol particles formed within the ML. The results suggest that in the boreal forest environment, NPF in the upper RL has an important contribution to the aerosol load in the boundary layer (BL).

scholarly journals Aerosol particle formation in the upper residual layer

2020 ◽  
Author(s):  
Janne Lampilahti ◽  
Katri Leino ◽  
Antti Manninen ◽  
Pyry Poutanen ◽  
Anna Franck ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Boreal Forest ◽  
Cloud Condensation Nuclei ◽  
Large Fraction ◽  
Aerosol Particles ◽  
Particle Formation ◽  
Residual Layer ◽  
Forest Environment ◽  
Near Surface

Abstract. According to current estimates, atmospheric new particle formation (NPF) produces a large fraction of aerosol particles and cloud condensation nuclei in the earth’s atmosphere, therefore having implications for health and climate. Despite recent advances, atmospheric NPF is still insufficiently understood in the upper parts of the boundary layer (BL). In addition, it is unclear how NPF in upper BL is related to the processes observed in the near-surface layer. The role of the topmost part of the residual layer (RL) in NPF is to a large extent unexplored. This paper presents new results from co-located airborne and ground-based measurements in a boreal forest environment, showing that many NPF events (∼42 %) appear to start in the upper RL. The freshly formed particles may be entrained into the growing mixed layer (ML) where they continue to grow in size, similar to the aerosol particles formed within the ML. The results suggest that in the boreal forest environment, NPF in the upper RL has an important contribution to the aerosol load in the BL.

scholarly journals Ventilation of a Mid-Size City under Stable Boundary Layer Conditions: A Simulation Using the LES Model PALM

Atmosphere ◽  
2021 ◽  
Vol 12 (3) ◽  
pp. 401
Author(s):  
Jonathan Biehl ◽  
Bastian Paas ◽  
Otto Klemm
Keyword(s):  
Boundary Layer ◽  
Stable Boundary Layer ◽  
Passive Scalar ◽  
City Center ◽  
Street Canyons ◽  
Stable Boundary ◽  
Northwest Germany ◽  
Stable Conditions ◽  
Les Model ◽  
The City

City centers have to cope with an increasing amount of air pollution. The supply of fresh air is crucial yet difficult to ensure, especially under stable conditions of the atmospheric boundary layer. This case study used the PArallelized Large eddy simulation (LES) Model PALM to investigate the wind field over an urban lake that had once been built as a designated fresh air corridor for the city center of Münster, northwest, Germany. The model initialization was performed using the main wind direction and stable boundary layer conditions as input. The initial wind and temperature profiles included a weak nocturnal low-level jet. By emitting a passive scalar at one point on top of a bridge, the dispersion of fresh air could be traced over the lake’s surface, within street canyons leading to the city center and within the urban boundary layer above. The concept of city ventilation was confirmed in principle, but the air took a direct route from the shore of the lake to the city center above a former river bed and its adjoining streets rather than through the street canyons. According to the dispersion of the passive scalar, half of the city center was supplied with fresh air originating from the lake. PALM proved to be a useful tool to study fresh air corridors under stable boundary layer conditions.

scholarly journals Thermal Submeso Motions in the Nocturnal Stable Boundary Layer. Part 2: Generating Mechanisms and Implications

2021 ◽  
Author(s):  
Lena Pfister ◽  
Karl Lapo ◽  
Larry Mahrt ◽  
Christoph K. Thomas
Keyword(s):  
Boundary Layer ◽  
Stable Boundary Layer ◽  
Side Wall ◽  
Cold Pool ◽  
Continuous Data ◽  
Valley Bottom ◽  
Near Surface ◽  
Cold Air ◽  
Stable Boundary ◽  
Surface Temperatures

AbstractIn the stable boundary layer, thermal submesofronts (TSFs) are detected during the Shallow Cold Pool experiment in the Colorado plains, Colorado, USA in 2012. The topography induces TSFs by forming two different air layers converging on the valley-side wall while being stacked vertically above the valley bottom. The warm-air layer is mechanically generated by lee turbulence that consistently elevates near-surface temperatures, while the cold-air layer is thermodynamically driven by radiative cooling and the corresponding cold-air drainage decreases near-surface temperatures. The semi-stationary TSFs can only be detected, tracked, and investigated in detail when using fibre-optic distributed sensing (FODS), as point observations miss TSFs most of the time. Neither the occurrence of TSFs nor the characteristics of each air layer are connected to a specific wind or thermal regime. However, each air layer is characterized by a specific relationship between the wind speed and the friction velocity. Accordingly, a single threshold separating different flow regimes within the boundary layer is an oversimplification, especially during the occurrence of TSFs. No local forcings or their combination could predict the occurrence of TSFs except that they are less likely to occur during stronger near-surface or synoptic-scale flow. While classical conceptualizations and techniques of the boundary layer fail in describing the formation of TSFs, the use of spatially continuous data obtained from FODS provide new insights. Future studies need to incorporate spatially continuous data in the horizontal and vertical planes, in addition to classic sensor networks of sonic anemometry and thermohygrometers to fully characterize and describe boundary-layer phenomena.

Tethered Balloon Observations Of The Nocturnal Stable Boundary Layer In A Valley

2000 ◽  
Vol 97 (1) ◽  
pp. 1-24 ◽  
Author(s):  
J. J. Holden ◽  
S. H. Derbyshire ◽  
S. E. Belcher
Keyword(s):  
Boundary Layer ◽  
Stable Boundary Layer ◽  
Tethered Balloon ◽  
Stable Boundary
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