sulfate aerosols
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2022 ◽  
Vol 578 ◽  
pp. 117299
Author(s):  
Ryu Uemura ◽  
Kosuke Masaka ◽  
Yoshinori Iizuka ◽  
Motohiro Hirabayashi ◽  
Hitoshi Matsui ◽  
...  

MAUSAM ◽  
2021 ◽  
Vol 52 (1) ◽  
pp. 229-244
Author(s):  
K. RUPA KUMAR ◽  
R. G. ASHRIT

The regional climatic impacts associated with global climatic change and their assessment are very important since agriculture, water resources, ecology etc., are all vulnerable to climatic changes on regional scale. Coupled Atmosphere-Ocean general circulation model (AOGCM) simulations provide a range of scenarios, which can be used, for the assessment of impacts and development of adaptive or mitigative strategies. Validation of the models against the observations and establishing the sensitivity to climate change forcing are essential before the model projections are used for assessment of possible impacts. Moreover model simulated climate projections are often of coarse resolution while the models used for impact assessment, (e.g. crop simulation models, or river runoff models etc.) operate on a higher spatial resolution. This spatial mismatch can be overcome by adopting an appropriate strategy of downscaling the GCM output.   This study examines two AOGCM (ECHAM4/OPYC3 and HadCM2) climate change simulations for their performance in the simulation of monsoon climate over India and the sensitivity of the simulated monsoon climate to transient changes in the atmospheric concentrations of greenhouse gases and sulfate aerosols. The results show that the two models simulate the gross features of climate over India reasonably well. However the inter-model differences in simulation of mean characteristics, sensitivity to forcing and in the simulation of climate change suggest need for caution. Further an empirical downscaling approach in used to assess the possibility of using GCM projections for preparation of regional climate change scenario for India.


MAUSAM ◽  
2021 ◽  
Vol 52 (1) ◽  
pp. 245-262
Author(s):  
M. LAL ◽  
SANJEEV K. SINGH

The response of the Asian summer monsoon to transient increases of greenhouse gases (GHGs) and sulfate aerosols in the Earth's atmosphere is examined using the data generated in numerical experiments with available coupled atmosphere-ocean global climate models (A-O GCMs). A comparison of observed and model-simulated trends in monthly mean near-surface temperature and rainfall over the region provides evidence of skill of the A-O GCMs in simulating the regional climatology. The potential role of the sulfate aerosols in obscuring the GHG- induced warming over the Indian subcontinent is discussed. Even though the simulated total seasonal rainfall over the Indian subcontinent during summer monsoon season is underestimated in most of the A-O GCMs, the year to year variability in simulated monsoon rainfall over the study region is found to be in fair agreement with the observed climatology.


2021 ◽  
Vol 9 ◽  
Author(s):  
Acharya Asutosh ◽  
Suvarna Fadnavis ◽  
M. Nuncio ◽  
Rolf Müller ◽  
Sarat C. Tripathy

The mechanisms behind Arctic warming and associated climate changes are difficult to discern. Also, the complex local processes and feedbacks like aerosol-cloud-climate interactions are yet to be quantified. Here, using the Community Earth System Model (CAM5) experiments, with emission enhancement of anthropogenic sulfate 1) five-fold globally, 2) ten-times over Asia, and 3) ten-times over Europe we show that regional emissions of sulfate aerosols alter seasonal warming over the Arctic, i.e., colder summer and warmer winter. European emissions play a dominant role in cooling during the summer season (0.7 K), while Asian emissions dominate the warming during the winter season (maximum ∼0.6 K) in the Arctic surface. The cooling/warming is associated with a negative/positive cloud radiative forcing. During the summer season increase in low–mid level clouds, induced by sulfate emissions, favours the solar dimming effect that reduces the downwelling radiation to the surface and thus leads to surface cooling. Warmer winters are associated with enhanced high-level clouds that induce a positive radiative forcing at the top of the atmosphere. This study points to the importance of international strategies being implemented to control sulfate emissions to combat air pollution. Such strategies will also affect the Arctic cooling/warming associated with a cloud radiative forcing caused by sulfate emission change.


2021 ◽  
Author(s):  
Frederic Bonou ◽  
Casimir Yelognisse Da-Allada ◽  
Ezinvi Baloïtcha ◽  
Eric Alamou ◽  
Eliezer Iboukoun Biao ◽  
...  

2021 ◽  
Author(s):  
Daniele Visioni ◽  
Simone Tilmes ◽  
Charles Bardeen ◽  
Michael Mills ◽  
Douglas G. MacMartin ◽  
...  

Abstract. Simulating the complex aerosol microphysical processes in a comprehensive Earth System Model can be very computationally intensive and therefore many models utilize a modal approach, where aerosol size distributions are represented by observations-derived lognormal functions. This approach has been shown to yield satisfactory results in a large array of applications, but there may be cases where the simplification in this approach may produce some shortcomings. In this work we show specific conditions under which the current approximations used in modal approaches might yield some incorrect answers. Using results from the Community Earth System Model v1 (CESM1) Geoengineering Large Ensemble (GLENS) project, we analyze the effects in the troposphere of a continuous increasing load of sulfate aerosols in the stratosphere, with the aim of counteracting the surface warming produced by non-mitigated increasing greenhouse gases concentration between 2020–2100. We show that the simulated results pertaining to the evolution of sea salt and dust aerosols in the upper troposphere are not realistic due to internal mixing assumptions in the modal aerosol treatment, which in this case reduces the size, and thus the settling velocities, of those particles and ultimately changes their mixing ratio below the tropopause. The unnatural increase of these aerosol species affects, in turn, the simulation of upper tropospheric ice formation, resulting in an increase in ice clouds that is not due to any meaningful physical mechanisms. While we show that this does not significantly affect the overall results of the simulations, we point to some areas where results should be interpreted with care in modeling simulations using similar approximations: in particular, the evolution of upper tropospheric clouds when large amount of sulfate is present in the stratosphere, as after a large explosive volcanic eruption or in similar stratospheric aerosol injection cases. Finally, we suggest that this could be avoided if sulfate aerosols in the coarse mode, the predominant species in these situation, are treated separately from other aerosol species in the model.


2021 ◽  
Vol 2 (1) ◽  
Author(s):  
Sergey Osipov ◽  
Georgiy Stenchikov ◽  
Kostas Tsigaridis ◽  
Allegra N. LeGrande ◽  
Susanne E. Bauer ◽  
...  

AbstractSupervolcano eruptions have occurred throughout Earth’s history and have major environmental impacts. These impacts are mostly associated with the attenuation of visible sunlight by stratospheric sulfate aerosols, which causes cooling and deceleration of the water cycle. Supereruptions have been assumed to cause so-called volcanic winters that act as primary evolutionary factors through ecosystem disruption and famine, however, winter conditions alone may not be sufficient to cause such disruption. Here we use Earth system model simulations to show that stratospheric sulfur emissions from the Toba supereruption 74,000 years ago caused severe stratospheric ozone loss through a radiation attenuation mechanism that only moderately depends on the emission magnitude. The Toba plume strongly inhibited oxygen photolysis, suppressing ozone formation in the tropics, where exceptionally depleted ozone conditions persisted for over a year. This effect, when combined with volcanic winter in the extra-tropics, can account for the impacts of supereruptions on ecosystems and humanity.


2021 ◽  
Author(s):  
Nick Gorkavyi ◽  
Nickolay Krotkov ◽  
Can Li ◽  
Leslie Lait ◽  
Peter Colarco ◽  
...  

Abstract. The June 21, 2019 eruption of the Raikoke volcano (Kuril Islands, Russia, 48°N, 153°E) produced significant amounts of volcanic aerosols (sulfate and ash) and sulfur dioxide (SO2) gas that penetrated into the lower stratosphere. The dispersed SO2 and sulfate aerosols in the stratosphere were still detectable by multiple satellite sensors for three months after the eruption. For this study of SO2 and aerosol clouds we use data obtained from two of the Ozone Mapping Profiler Suite (OMPS) sensors on the Suomi National Polar-orbiting Partnership (SNPP) satellite: total column SO2 from the Nadir Mapper (NM) and aerosol extinction profiles from the Limb Profiler (LP) as well as other satellite data sets. The LP standard aerosol extinction product at 674 nm has been re-processed with an adjustment correcting for limb viewing geometry effects. It was shown that the amount of SO2 decreases with a characteristic period of 8–18 days and the peak of sulfate aerosol recorded at a wavelength of 674 nm lags the initial peak of SO2 by 1.5 months. Using satellite observations and a trajectory model, we examined the dynamics of unusual atmospheric feature that was observed, a stratospheric coherent circular cloud (CCC) of SO2 and aerosol from July 18 to September 22, 2019.


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