Optical Nuclear Spin Polarization of Divacancies in SiC

2016 ◽  
Vol 858 ◽  
pp. 287-290
Author(s):  
Viktor Ivády ◽  
Krisztián Szász ◽  
Abram L. Falk ◽  
Paul V. Klimov ◽  
David J. Christle ◽  
...  

We demonstrate optically pumped dynamic nuclear polarization (DNP) of 29Si nuclear spins that are strongly coupled to paramagnetic color centers in 4H- and 6H-SiC. We observe 99%±1% degree of polarization. By combining ab initio theory with the experimental identification of the color centers’ optically excited states, we quantitatively model how the polarization derives from hyperfine-mediated level anticrossings. In addition, we developed a general model for these optical DNP processes that allows the effects of many microscopic processes to be integrated. Applying this theory, we gain a deeper insight into dynamic nuclear spin polarization. In particular, our findings show that the defect electron spin coherence times and excited state lifetimes are crucial factors in the entire DNP process. These results lay a foundation for SiC-based quantum memories, nuclear gyroscopes, and hyperpolarized probes for magnetic resonance imaging.

2009 ◽  
Vol 23 (12n13) ◽  
pp. 2737-2738
Author(s):  
YOSHIRO HIRAYAMA

Nuclear magnetic resonance (NMR) is widely used in the physical, chemical, and biological sciences. However, conventional NMR techniques based on induction-detection have drawbacks of low-sensitivity and the need of a relatively large sample. It is not suitable to investigate single or double layers (or their nanostructure), which is essential in studying quantum Hall (QH) effects. In this presentation, I discussed a resistively-detected technique to overcome the low-sensitivity limitation of conventional NMR and its application to QH systems. Resistively-detected nuclear-spin-based measurements rely on enhanced interactions between electron and nuclear spins at the degenerate point of different electron-spin states. For example, at the ν = 2/3 degenerate point in a AlGaAs / GaAs system,1–3 nuclear-spin polarization far beyond the thermal equilibrium is generated using current flow (dynamic nuclear-spin polarization). Moreover, nuclear-spin polarization can be detected as enhanced resistance, which is proportional to the magnetization, Mz, of nuclear spins.2 It should be stressed that the special states of ν = 2/3 are needed for dynamic nuclear-spin polarization and Mz detection, but we can apply NMR spectrum and nuclear-spin relaxation (T1 time) measurements for any state we want to estimate. These nuclear-spin-based measurements were successfully applied to characterize QH systems, especially their electron-spin features, using single and double layer systems where characteristics are controlled electrically by the gate biases. For a single layer, we could clarify skyrmion,2 spin-polarization of composite fermion,4 and enhanced spin-orbit interactions in a strongly asymmetric confinement.5 Exciting phases, like a canted antiferromagnetic phase, were studied in a double layer QH system with a total filling factor of 2 (Refs. 6, 7). The low-frequency mode was sensitively detected by monitoring T1, reflecting correlated electron spin features.7 The clear observations of the characteristics, which are difficult to detect in conventional transport and optical measurements, make nuclear-spin-based measurement combined with resistance-detection a versatile and powerful tool for studying QH physics. Possible extensions of such measurements to semiconductor nanosystems were also discussed. The experiments discussed here were mainly carried out at NTT Basic Research Laboratories in collaboration with K. Muraki, N. Kumada, K. Takashina, K. Hashimoto, S. Watanabe and G. Yusa. Note from Publisher: This article contains the abstract only.


Nanoscale ◽  
2014 ◽  
Vol 6 (17) ◽  
pp. 10134-10139 ◽  
Author(s):  
Gang-Qin Liu ◽  
Qian-Qing Jiang ◽  
Yan-Chun Chang ◽  
Dong-Qi Liu ◽  
Wu-Xia Li ◽  
...  

Centre spin coherence is well protected by preparing its bath spins state, even with unknown hyperfine interactions.


2011 ◽  
Vol 10 (11) ◽  
pp. 844-848 ◽  
Author(s):  
M. N. Makhonin ◽  
K. V. Kavokin ◽  
P. Senellart ◽  
A. Lemaître ◽  
A. J. Ramsay ◽  
...  

2009 ◽  
Vol 23 (12n13) ◽  
pp. 2755-2759 ◽  
Author(s):  
DAISUKE FUKUOKA ◽  
NAOKI TANAKA ◽  
KENICHI OTO ◽  
KIYOFUMI MURO ◽  
YOSHIRO HIRAYAMA ◽  
...  

The dynamics between electron and nuclear spins in quantum Hall regime is investigated by a time-resolved Kerr rotation (TRKR) spectroscopy carried down in tilted-field geometry. The spin-flip energy varies almost linearly with the applied magnetic field under the nuclear spin depolarizing radio frequency field and the helicity modulation of circularly polarized pump, while the spin-flip energy obtained under a circularly polarized pump deviates from linearly behavior. This deviation is ascribed to the Overhauser shift due to dynamic nuclear spin polarization (DNP). The DNP depends markedly on the filling factor and present peaks at even filling factors. These results can be well explained by a simple model based on the detailed balance between electron and nuclear spins.


Author(s):  
M. M. Glazov

The transfer of nonequilibrium spin polarization between the electron and nuclear subsystems is studied in detail. Usually, a thermal orientation of nuclei in magnetic field is negligible due to their small magnetic moments, but if electron spins are optically oriented, efficient nuclear spin polarization can occur. The microscopic approach to the dynamical nuclear polarization effect based on the kinetic equation method, along with a phenomenological but very powerful description of dynamical nuclear polarization in terms of the nuclear spin temperature concept is given. In this way, one can account for the interaction between neighbouring nuclei without solving a complex many-body problem. The hyperfine interaction also induces the feedback of polarized nuclei on the electron spin system giving rise to a number of nonlinear effects: bistability of nuclear spin polarization and anomalous Hanle effect, dragging and locking of optical resonances in quantum dots. Theory is illustrated by experimental data on dynamical nuclear polarization.


2016 ◽  
Vol 93 (8) ◽  
Author(s):  
F. Heisterkamp ◽  
E. Kirstein ◽  
A. Greilich ◽  
E. A. Zhukov ◽  
T. Kazimierczuk ◽  
...  

1982 ◽  
Vol 104 (22) ◽  
pp. 5878-5883 ◽  
Author(s):  
Richard S. Hutton ◽  
Heinz D. Roth ◽  
Marcia L. Manion Schilling ◽  
Anthony M. Trozzolo ◽  
Thomas M. Leslie

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