Review of Characterization of Arctic mixed-phase cloud properties

2017 ◽  
Author(s):  
Anonymous
Keyword(s):  
2020 ◽  
Vol 12 (23) ◽  
pp. 3946
Author(s):  
Pasquale Sellitto ◽  
Silvia Bucci ◽  
Bernard Legras

Clouds in the tropics have an important role in the energy budget, atmospheric circulation, humidity, and composition of the tropical-to-global upper-troposphere–lower-stratosphere. Due to its non-sun-synchronous orbit, the Cloud–Aerosol Transport System (CATS) onboard the International Space Station (ISS) provided novel information on clouds from space in terms of overpass time in the period of 2015–2017. In this paper, we provide a seasonally resolved comparison of CATS characterization of high clouds (between 13 and 18 km altitude) in the tropics with well-established CALIPSO (Cloud–Aerosol Lidar and Infrared Pathfinder Satellite Observation) data, both in terms of clouds’ occurrence and cloud optical properties (optical depth). Despite the fact that cloud statistics for CATS and CALIOP are generated using intrinsically different local overpass times, the characterization of high clouds occurrence and optical properties in the tropics with the two instruments is very similar. Observations from CATS underestimate clouds occurrence (up to 80%, at 18 km) and overestimate the occurrence of very thick clouds (up to 100% for optically very thick clouds, at 18 km) at higher altitudes. Thus, the description of stratospheric overshoots with CATS and CALIOP might be different. While this study hints at the consistency of CATS and CALIOP clouds characterizaton, the small differences highlighted in this work should be taken into account when using CATS for estimating cloud properties and their variability in the tropics.


2021 ◽  
Author(s):  
Minghui Zhang ◽  
Amina Khaled ◽  
Pierre Amato ◽  
Anne-Marie Delort ◽  
Barbara Ervens

<p>Primary biological aerosol particles (PBAPs) play an important role in mixed-phase clouds as they nucleate ice even at temperatures of T > -10 °C. Current parameterizations of PBAP ice nucleation are based on ice nucleation active surface site (INAS) densities that are derived from freezing experiments. However, only a small fraction of the PBAP surface is responsible for their ice nucleation activity, such as proteins of bacteria cells, fungal spores, pollen polysaccharides and other (unidentified) macromolecules. Based on literature data, we refine the INAS density parameterizations by further parameters:</p><p>1) We demonstrate that the ice nucleation activity of such individual macromolecules is much higher than that of PBAPs. It can be shown that INAS of PBAPs can be scaled by the surface fraction of these ice-nucleating molecules.</p><p>2) Previous studies suggested that ice nucleation activity tends to be higher for larger macromolecules and their aggregates. We show that these trends hold true for various groups of macromolecules that comprise PBAPs.</p><p>Based on these trends, we suggest a more refined parameterization for ice-nucleating macromolecules in different types of PBAPs and even for different species of bacteria, fungi, and pollen. This new parameterization can be considered a step towards a molecular-based approach to predict the ice nucleation activity of the macromolecules in PBAPs based on their biological and chemical properties.</p><p>We implement both the traditional INAS parameterization for complete PBAPs and our parameterization for individual molecules in an adiabatic cloud parcel model. The extent will be discussed to which the two parameterizations result in different cloud properties of mixed-phase clouds.</p>


2019 ◽  
Vol 33 (36) ◽  
pp. 1950461 ◽  
Author(s):  
Yan Qi ◽  
Bingqian Bi ◽  
Yilin Yan ◽  
Lecheng Tian

In this study, a leaf-like [Formula: see text] mixed phase nanosheets array was successfully prepared by anodization. XRD, EDS, and XPS analysis confirmed the formation of [Formula: see text] mixed phase nanostructures. SEM images indicate that the fabricated [Formula: see text] mixed phase nanosheets almost grow vertically on the substrate. The average height of nanosheets is approximately 500 nm. The optical absorption of the mixed phase covers the entire wavelength region of visible light and a little part of the near-infrared region of short wavelength.


2017 ◽  
Author(s):  
Micael A. Cecchini ◽  
Luiz A. T. Machado ◽  
Manfred Wendisch ◽  
Anja Costa ◽  
Martina Krämer ◽  
...  

Abstract. The behavior of tropical clouds remains a major open scientific question, given that the associated phys-ics is not well represented by models. One challenge is to realistically reproduce cloud droplet size dis-tributions (DSD) and their evolution over time and space. Many applications, not limited to models, use the Gamma function to represent DSDs. However, there is almost no study dedicated to understanding the phase space of this function, which is given by the three parameters that define the DSD intercept, shape, and curvature. Gamma phase space may provide a common framework for parameterizations and inter-comparisons. Here, we introduce the phase-space approach and its characteristics, focusing on warm-phase microphysical cloud properties and the transition to the mixed-phase layer. We show that trajectories in this phase space can represent DSD evolution and can be related to growth processes. Condensational and collisional growth may be interpreted as pseudo-forces that induce displacements in opposite directions within the phase space. The actually observed movements in the phase space are a result of the combination of such pseudo-forces. Additionally, aerosol effects can be evaluated given their significant impact on DSDs. The DSDs associated with liquid droplets that favor cloud glaciation can be delimited in the phase space, which can help models to adequately predict the transition to the mixed phase. We also consider possible ways to constrain the DSD in two-moment bulk microphysics schemes, where the relative dispersion parameter of the DSD can play a significant role. Overall, the Gamma phase-space approach can be an invaluable tool for studying cloud microphysical evolution and can be readily applied in many scenarios that rely on Gamma DSDs.


1993 ◽  
Vol 60 (1-3) ◽  
pp. 502-505 ◽  
Author(s):  
M.Z. Karim ◽  
D.C. Cameron ◽  
M.S.J. Hashmi
Keyword(s):  

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