scholarly journals Physical and optical properties of 2010 Eyjafjallajökull volcanic eruption aerosol: ground-based, LIDAR and airborne measurements in France

2011 ◽  
Vol 11 (9) ◽  
pp. 24631-24670 ◽  
Author(s):  
M. Hervo ◽  
B. Quennehen ◽  
N. I. Kristiansen ◽  
J. Boulon ◽  
A. Stohl ◽  
...  
Keyword(s):  
Remote Sensing ◽  
Boundary Layer ◽  
Optical Properties ◽  
Mass Concentration ◽  
Dispersion Model ◽  
Free Troposphere ◽  
Data Set ◽  
Model Simulations ◽  
Ash Cloud

Abstract. During the Eyjafjallajökull eruption (14 April to 24 May 2010), the volcanic aerosol cloud was observed across Europe by several airborne in-situ and ground-based remote-sensing instruments. On 18 and 19 May, layers of depolarizing particles (i.e. non-spherical particles) were detected in the free troposphere above the Puy de Dôme station, (France) with a Rayleigh-Mie LIDAR emitting at a wavelength of 355 nm, with parallel and crossed polarization channels. These layers in the free troposphere (FT) were also well captured by simulations with the Lagrangian particle dispersion model FLEXPART, which furthermore showed that the ash was eventually entrained into the planetary boundary layer (PBL). Indeed, the ash cloud was then detected and characterized with a comprehensive set of in-situ instruments at the Puy de Dôme station (PdD). In agreement with the FLEXPART simulation, up to 65 μg m−3 of particle mass and 2.2 ppb of SO2 were measured at PdD, corresponding to concentrations higher than the 95 percentile of 2 years of measurements at PdD. Moreover, the number concentration of particles increased to 24 000 cm−3, mainly in the submicronic mode, but a supermicronic mode was also detected at 2 μm. The resulting optical properties of the ash aerosol were characterized by a low Ångström exponent (1.1), showing the dominance of supermicronic particles. For the first time to our knowledge, the combination of in-situ optical and physical characterization of the volcanic ash allowed the calculation of the mass-to-extinction ratio (η) with no assumptions on the aerosol density, which was found to be significantly different from the background boundary layer aerosol (max: 1.42 g m−2 as opposed to 0.27 ± 0.03 g m−2). Using this ratio, ash mass concentration in the volcanic plume derived from LIDAR measurements was found to be 700 ± 25 μg m−3 when the plume was located in the FT (3000 m a.s.l. – above sea level). This ratio could also be used to retrieve an aerosol mass concentration of 523 ± 54 μg m−3 on 19 April, when LIDAR observations detected the ash cloud at 3000 m a.s.l. in correspondence with model simulations (FLEXPART). On 22 April, another ash plume entered the BL, and although it was more diluted than during the May episode, the French research aircraft ATR42 that passed over Clermont-Ferrand in the PBL confirmed the presence of particles with a supermicronic mode, again centred on a diameter of 2 μm. This data set combining airborne, ground-based and remote sensing observations with dispersion model simulations shows an overall very good coherence during the volcanic eruption period, which allows a good confidence in the characteristics of the ash particles that can be derived from this unique data set.

scholarly journals Physical and optical properties of 2010 Eyjafjallajökull volcanic eruption aerosol: ground-based, Lidar and airborne measurements in France

2012 ◽  
Vol 12 (4) ◽  
pp. 1721-1736 ◽  
Author(s):  
M. Hervo ◽  
B. Quennehen ◽  
N. I. Kristiansen ◽  
J. Boulon ◽  
A. Stohl ◽  
...  
Keyword(s):  
Remote Sensing ◽  
Boundary Layer ◽  
Mass Concentration ◽  
Dispersion Model ◽  
Extinction Ratio ◽  
Free Troposphere ◽  
Data Set ◽  
Model Simulations ◽  
Ash Cloud

Abstract. During the Eyjafjallajökull eruption (14 April to 24 May 2010), the volcanic aerosol cloud was observed across Europe by several airborne in situ and ground-based remote-sensing instruments. On 18 and 19 May, layers of depolarizing particles (i.e. non-spherical particles) were detected in the free troposphere above the Puy de Dôme station, (PdD, France) with a Rayleigh-Mie LIDAR emitting at a wavelength of 355 nm, with parallel and crossed polarization channels. These layers in the free troposphere (FT) were also well captured by simulations with the Lagrangian particle dispersion model FLEXPART, which furthermore showed that the ash was eventually entrained into the planetary boundary layer (PBL). Indeed, the ash cloud was then detected and characterized with a comprehensive set of in situ instruments at the Puy de Dôme station (PdD). In agreement with the FLEXPART simulation, up to 65 μg m−3 of particle mass and 2.2 ppb of SO2 were measured at PdD, corresponding to concentrations higher than the 95 percentile of 2 yr of measurements at PdD. Moreover, the number concentration of particles increased to 24 000 cm−3, mainly in the submicronic mode, but a supermicronic mode was also detected with a modal diameter of 2 μm. The resulting optical properties of the ash aerosol were characterized by a low scattering Ångström exponent (0.98), showing the presence of supermicronic particles. For the first time to our knowledge, the combination of in situ optical and physical characterization of the volcanic ash allowed the calculation of the mass-to-extinction ratio (η) with no assumptions on the aerosol density. The mass-to-extinction ratio was found to be significantly different from the background boundary layer aerosol (max: 1.57 g m−2 as opposed to 0.33 ± 0.03 g m−2). Using this ratio, ash mass concentration in the volcanic plume derived from LIDAR measurements was found to be 655 ± 23 μg m−3 when the plume was located in the FT (3000 m above the sea level – a.s.l.). This ratio could also be used to retrieve an aerosol mass concentration of 579 ± 60 μg m−3 on 19 April, when LIDAR observations detected the ash cloud at 3000 m a.s.l. in correspondence with model simulations (FLEXPART). On 22 April, another ash plume entered the BL, and although it was more diluted than during the May episode, the French research aircraft ATR42 that passed over Clermont-Ferrand in the PBL confirmed the presence of particles with a supermicronic mode, again with a modal diameter at 2 μm. This data set combining airborne, ground-based and remote sensing observations with dispersion model simulations shows an overall very good coherence during the volcanic eruption period, which allows a good confidence in the characteristics of the ash particles that can be derived from this unique data set.

scholarly journals Aircraft validation of Aura Tropospheric Emission Spectrometer retrievals of HDO / H<sub>2</sub>O

2014 ◽  
Vol 7 (9) ◽  
pp. 3127-3138 ◽  
Author(s):  
R. L. Herman ◽  
J. E. Cherry ◽  
J. Young ◽  
J. M. Welker ◽  
D. Noone ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Water Vapor ◽  
Standard Deviation ◽  
Lower Troposphere ◽  
Temporal Variations ◽  
Observation Error ◽  
Free Troposphere ◽  
Data Set ◽  
Airborne Measurements

Abstract. The EOS (Earth Observing System) Aura Tropospheric Emission Spectrometer (TES) retrieves the atmospheric HDO / H2O ratio in the mid-to-lower troposphere as well as the planetary boundary layer. TES observations of water vapor and the HDO isotopologue have been compared with nearly coincident in situ airborne measurements for direct validation of the TES products. The field measurements were made with a commercially available Picarro L1115-i isotopic water analyzer on aircraft over the Alaskan interior boreal forest during the three summers of 2011 to 2013. TES special observations were utilized in these comparisons. The TES averaging kernels and a priori constraints have been applied to the in situ data, using version 5 (V005) of the TES data. TES calculated errors are compared with the standard deviation (1σ) of scan-to-scan variability to check consistency with the TES observation error. Spatial and temporal variations are assessed from the in situ aircraft measurements. It is found that the standard deviation of scan-to-scan variability of TES δD is ±34.1‰ in the boundary layer and ± 26.5‰ in the free troposphere. This scan-to-scan variability is consistent with the TES estimated error (observation error) of 10–18‰ after accounting for the atmospheric variations along the TES track of ±16‰ in the boundary layer, increasing to ±30‰ in the free troposphere observed by the aircraft in situ measurements. We estimate that TES V005 δD is biased high by an amount that decreases with pressure: approximately +123‰ at 1000 hPa, +98‰ in the boundary layer and +37‰ in the free troposphere. The uncertainty in this bias estimate is ±20‰. A correction for this bias has been applied to the TES HDO Lite Product data set. After bias correction, we show that TES has accurate sensitivity to water vapor isotopologues in the boundary layer.

scholarly journals Aerosol optical and microphysical retrievals from a hybrid multiwavelength lidar data set – DISCOVER-AQ 2011

2014 ◽  
Vol 7 (9) ◽  
pp. 3095-3112 ◽  
Author(s):  
P. Sawamura ◽  
D. Müller ◽  
R. M. Hoff ◽  
C. A. Hostetler ◽  
R. A. Ferrare ◽  
...  
Keyword(s):  
Remote Sensing ◽  
In Situ Measurements ◽  
Index Of Refraction ◽  
High Spectral Resolution ◽  
Lidar Data ◽  
Data Set ◽  
Microphysical Properties ◽  
Lidar Measurements ◽  
Multiwavelength Lidar

Abstract. Retrievals of aerosol microphysical properties (effective radius, volume and surface-area concentrations) and aerosol optical properties (complex index of refraction and single-scattering albedo) were obtained from a hybrid multiwavelength lidar data set for the first time. In July 2011, in the Baltimore–Washington DC region, synergistic profiling of optical and microphysical properties of aerosols with both airborne (in situ and remote sensing) and ground-based remote sensing systems was performed during the first deployment of DISCOVER-AQ. The hybrid multiwavelength lidar data set combines ground-based elastic backscatter lidar measurements at 355 nm with airborne High-Spectral-Resolution Lidar (HSRL) measurements at 532 nm and elastic backscatter lidar measurements at 1064 nm that were obtained less than 5 km apart from each other. This was the first study in which optical and microphysical retrievals from lidar were obtained during the day and directly compared to AERONET and in situ measurements for 11 cases. Good agreement was observed between lidar and AERONET retrievals. Larger discrepancies were observed between lidar retrievals and in situ measurements obtained by the aircraft and aerosol hygroscopic effects are believed to be the main factor in such discrepancies.

scholarly journals Estudo do ciclo diário da Camada Limite Planetária durante a estação cChuvosa da Amazônia (GOAmazon 2014/15)

2018 ◽  
Vol 40 ◽  
pp. 63 ◽  
Author(s):  
Rayonil Gomes Carneiro ◽  
Alice Henkes ◽  
Gilberto Fisch ◽  
Camilla Kassar Borges
Keyword(s):  
Remote Sensing ◽  
Boundary Layer ◽  
Planetary Boundary Layer ◽  
Remote Sensing Data ◽  
Great Depth ◽  
Wet Season ◽  
Daily Cycle ◽  
Convective Boundary ◽  
In Situ Observations

In the present study, the evolution the diurnal cycle of planetary boundary layer in the wet season at Amazon region during a period of intense observations carried out in the GOAmazon Project 2014/2015 (Green Ocean Amazon).The analysis includes radiosonde and remote sensing data. In general case, the results of the daily cycle in the wet season indicate a Nocturnal boundary layer with a small oscillation in its depth and with a tardy erosion. The convective boundary layer did not present great depth, responding to the low values of sensible heat of the wet season. A comparison between the different techniques(in situ observations and remote sensing)  for estimating the planetary boundary layer is also presented.

scholarly journals An Algorithm to Estimate Suspended Particulate Matter Concentrations and Associated Uncertainties from Remote Sensing Reflectance in Coastal Environments

2020 ◽  
Vol 12 (13) ◽  
pp. 2172 ◽  
Author(s):  
Juliana Tavora ◽  
Emmanuel Boss ◽  
David Doxaran ◽  
Paul Hill
Keyword(s):  
Remote Sensing ◽  
Optical Properties ◽  
Particulate Matter ◽  
Suspended Particulate Matter ◽  
Ocean Color ◽  
Major Constituent ◽  
Coastal Environments ◽  
Suspended Particulate ◽  
Spm Concentration

Suspended Particulate Matter (SPM) is a major constituent in coastal waters, involved in processes such as light attenuation, pollutant propagation, and waterways blockage. The spatial distribution of SPM is an indicator of deposition and erosion patterns in estuaries and coastal zones and a necessary input to estimate the material fluxes from the land through rivers to the sea. In-situ methods to estimate SPM provide limited spatial data in comparison to the coverage that can be obtained remotely. Ocean color remote sensing complements field measurements by providing estimates of the spatial distributions of surface SPM concentration in natural waters, with high spatial and temporal resolution. Existing methods to obtain SPM from remote sensing vary between purely empirical ones to those that are based on radiative transfer theory together with empirical inputs regarding the optical properties of SPM. Most algorithms use a single satellite band that is switched to other bands for different ranges of turbidity. The necessity to switch bands is due to the saturation of reflectance as SPM concentration increases. Here we propose a multi-band approach for SPM retrievals that also provides an estimate of uncertainty, where the latter is based on both uncertainties in reflectance and in the assumed optical properties of SPM. The approach proposed is general and can be applied to any ocean color sensor or in-situ radiometer system with red and near-infra-red bands. We apply it to six globally distributed in-situ datasets of spectral water reflectance and SPM measurements over a wide range of SPM concentrations collected in estuaries and coastal environments (the focus regions of our study). Results show good performance for SPM retrieval at all ranges of concentration. As with all algorithms, better performance may be achieved by constraining empirical assumptions to specific environments. To demonstrate the flexibility of the algorithm we apply it to a remote sensing scene from an environment with highly variable sediment concentrations.

scholarly journals Lower-free tropospheric ozone dial measurements over Athens, Greece

2018 ◽  
Vol 176 ◽  
pp. 05025 ◽  
Author(s):  
Michail Mytilinaios ◽  
Alexandros Papayannis ◽  
Georgios Tsaknakis
Keyword(s):  
Remote Sensing ◽  
Boundary Layer ◽  
Tropospheric Ozone ◽  
Vertical Profile ◽  
Stimulated Raman Scattering ◽  
Laser Wavelength ◽  
Free Troposphere ◽  
Differential Absorption ◽  
Raman Cell ◽  
Laser Remote Sensing

A compact ozone differential absorption lidar (DIAL) was implemented at the Laboratory of Laser Remote Sensing of the National Technical University of Athens (NTUA), in Athens, Greece. The DIAL system is based on a Nd:YAG laser emitting at 266 nm. A high-pressure Raman cell, filled with D2, was used to generate the λON and λOFF laser wavelength pairs (i.e., 266-289 nm and 289-316 nm, respectively) based on the Stimulated Raman Scattering (SRS) effect. The system was run during daytime and nighttime conditions to obtain the vertical profile of tropospheric ozone in the Planetary Boundary Layer (PBL) and the adjacent free troposphere.

scholarly journals Factors that influence surface PM<sub>2.5</sub> values inferred from satellite observations: perspective gained for the US Baltimore–Washington metropolitan area during DISCOVER-AQ

2014 ◽  
Vol 14 (4) ◽  
pp. 2139-2153 ◽  
Author(s):  
S. Crumeyrolle ◽  
G. Chen ◽  
L. Ziemba ◽  
A. Beyersdorf ◽  
L. Thornhill ◽  
...  
Keyword(s):  
Remote Sensing ◽  
Metropolitan Area ◽  
Scattering Coefficient ◽  
Data Set ◽  
Ambient Relative Humidity ◽  
Microphysical Properties ◽  
The Us ◽  
Dry Conditions ◽  
The Impact

Abstract. During the NASA DISCOVER-AQ campaign over the US Baltimore, MD–Washington, D.C., metropolitan area in July 2011, the NASA P-3B aircraft performed extensive profiling of aerosol optical, chemical, and microphysical properties. These in situ profiles were coincident with ground-based remote sensing (AERONET) and in situ (PM2.5) measurements. Here, we use this data set to study the correlation between the PM2.5 observations at the surface and the column integrated measurements. Aerosol optical depth (AOD550 nm) calculated with the extinction (550 nm) measured during the in situ profiles was found to be strongly correlated with the volume of aerosols present in the boundary layer (BL). Despite the strong correlation, some variability remains, and we find that the presence of aerosol layers above the BL (in the buffer layer – BuL) introduces significant uncertainties in PM2.5 estimates based on column-integrated measurements (overestimation of PM2.5 by a factor of 5). This suggests that the use of active remote sensing techniques would dramatically improve air quality retrievals. Indeed, the relationship between the AOD550 nm and the PM2.5 is strongly improved by accounting for the aerosol present in and above the BL (i.e., integrating the aerosol loading from the surface to the top of the BuL). Since more than 15% of the AOD values observed during DISCOVER-AQ are dominated by aerosol water uptake, the f(RH)amb (ratio of scattering coefficient at ambient relative humidity (RH) to scattering coefficient at low RH; see Sect. 3.2) is used to study the impact of the aerosol hygroscopicity on the PM2.5 retrievals. The results indicate that PM2.5 can be predicted within a factor up to 2 even when the vertical variability of the f(RH)amb is assumed to be negligible. Moreover, f(RH = 80%) and RH measurements performed at the ground may be used to estimate the f(RH)amb during dry conditions (RHBL < 55%).

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