scholarly journals Validation of six years of TES tropospheric ozone retrievals with ozonesonde measurements: implications for spatial patterns and temporal stability in the bias

2013 ◽  
Vol 6 (5) ◽  
pp. 1413-1423 ◽  
Author(s):  
W. W. Verstraeten ◽  
K. F. Boersma ◽  
J. Zörner ◽  
M. A. F. Allaart ◽  
K. W. Bowman ◽  
...  
Keyword(s):  
Degrees Of Freedom ◽  
A Priori ◽  
Temporal Stability ◽  
Lower Troposphere ◽  
Temporal Variations ◽  
Upper Troposphere ◽  
The World ◽  
The Difference ◽  
The Tropics

Abstract. In this analysis, Tropospheric Emission Spectrometer (TES) V004 nadir ozone (O3) profiles are validated with more than 4400 coinciding ozonesonde measurements taken across the world from the World Ozone and Ultraviolet Radiation Data Centre (WOUDC) during the period 2005–2010. The TES observation operator was applied to the sonde data to ensure a consistent comparison between TES and ozonesonde data, i.e. without the influence of the a priori O3 profile needed to regulate the retrieval. Generally, TES V004 O3 retrievals are biased high by 2–7 ppbv (7–15%) in the troposphere, consistent with validation results from earlier studies. Because of two degrees of freedom for signal in the troposphere, we can distinguish between upper and lower troposphere mean biases, respectively ranging from −0.4 to +13.3 ppbv for the upper troposphere and +3.9 to +6.0 ppbv for the lower troposphere. Focusing on the 464 hPa retrieval level, broadly representative of the free tropospheric O3, we find differences in the TES biases for the tropics (+3 ppbv, +7%), sub-tropics (+5 ppbv, +11%), and northern (+7 ppbv, +13%) and southern mid-latitudes (+4 ppbv, +10%). The relatively long-term record (6 yr) of TES–ozonesonde comparisons allowed us to quantify temporal variations in TES biases at 464 hPa. We find that there are no discernable biases in each of these latitudinal bands; temporal variations in the bias are typically within the uncertainty of the difference between TES and ozonesondes. Establishing these bias patterns is important in order to make meaningful use of TES O3 data in applications such as model evaluation, trend analysis, or data assimilation.

scholarly journals Validation of six years of TES tropospheric ozone retrievals with ozonesonde measurements: implications for spatial patterns and temporal stability in the TES bias

2013 ◽  
Vol 6 (1) ◽  
pp. 1239-1267 ◽  
Author(s):  
W. W. Verstraeten ◽  
K. F. Boersma ◽  
J. Zörner ◽  
M. A. F. Allaart ◽  
K. W. Bowman ◽  
...  
Keyword(s):  
Tropospheric Ozone ◽  
Degrees Of Freedom ◽  
A Priori ◽  
Temporal Stability ◽  
Lower Troposphere ◽  
Temporal Variations ◽  
The World ◽  
The Difference ◽  
The Tropics

Abstract. In this analysis, Tropospheric Emission Spectrometer (TES) V004 nadir ozone profiles are validated with more than 4400 coinciding ozonesonde measurements taken across the world from the World Ozone and Ultraviolet Radiation Data Centre (WOUDC) during the period 2005–2010. The TES observation operator was applied to the sonde data to ensure a consistent comparison between TES and ozonesonde data, i.e. without the influence of the a priori O3 profile needed to regulate the retrieval. Generally, TES V004 ozone retrievals are biased high by 2–7 ppbv in the troposphere, consistent with validation results from earlier studies. Because of two degrees of freedom for signal in the troposphere, we can distinguish between upper and lower troposphere mean biases, respectively ranging from −0.4 to +13.3 ppbv for the upper troposphere and +3.9 to +6.0 ppbv for the lower troposphere. Focusing on the 464 hPa retrieval level, broadly representative for free tropospheric ozone, we find differences in the TES biases for the Tropics (+3 ppbv), sub-tropics (+5 ppbv), and northern (+7 ppbv) and southern mid-latitudes (+4 ppbv). The relatively long-term record (6 yr) of TES-ozonesonde comparisons, allowed us to quantify temporal variations in TES biases in free tropospheric ozone, at 464 hPa. We find that there are no discernable biases in each of these latitudinal bands; temporal variations in the bias are typically within the uncertainty of the difference between TES and ozone-sondes. Establishing these bias patterns is important in order to make meaningful use of TES O3 data in applications such as model evaluation, trend analysis, or data assimilation.

scholarly journals Validation of the IASI FORLI/Eumetsat ozone products using satellite (GOME-2), ground-based (Brewer-Dobson, SAOZ) and ozonesonde measurements

2018 ◽  
Author(s):  
Anne Boynard ◽  
Daniel Hurtmans ◽  
Katerina Garane ◽  
Florence Goutail ◽  
Juliette Hadji-Lazaro ◽  
...  
Keyword(s):  
A Priori ◽  
Long Term Stability ◽  
Comparison Results ◽  
Independent Observations ◽  
Mean Differences ◽  
A Priori Uncertainty ◽  
The Tropics ◽  
Global Mean

Abstract. This paper assesses the quality of IASI/Metop-A (IASI-A) and IASI/Metop-B (IASI-B) ozone (O3) products (total and partial O3 columns) retrieved with the Fast Optimal Retrievals on Layers for IASI Ozone (FORLI-O3) v20151001 software for nine years (2008–2017) through an extensive inter-comparison and validation exercise using independent observations (satellite, ground-based and ozonesonde). IASI-A and IASI-B Total O3 Columns (TOCs) are generally consistent, with a global mean difference less than 0.3 % for both day- and nighttime measurements, IASI-A being slightly higher than IASI-B. A global difference less than 2.4 % is found for the tropospheric (TROPO) O3 column product (IASI-A being lower than IASI-B), which is partly due to a temporary issue related to IASI-A viewing angle in 2015. Our validation shows that IASI-A and IASI-B TOCs are consistent with GOME-2, Dobson, Brewer and SAOZ retrieved ones, with global mean differences in the range 0.1–2 % depending on the instruments. The IASI-A and ground-based TOC comparison for the period 2008–July 2017 shows good long-term stability (negative trends within 3 % decade−1). The comparison results between IASI-A and IASI-B against smoothed ozonesonde partial O3 columns vary in altitude and latitude, with maximum standard deviation for the 300–150 hPa column (20–40 %) due to strong ozone variability and a priori uncertainty. The worst agreement with the ozonesondes and with UV-vis retrieved TOC [satellite and ground] is found at the southern high latitudes. Compared to ozonesonde data, IASI-A and IASI-B O3 products overestimate the O3 abundance in the stratosphere (up to 20 % for the 150–25 hPa column) and underestimates the O3 abundance in the troposphere (within 10 % for the mid-latitudes and ~ 18 % for the tropics). Based on the period 2011–2016, non-significant drift is found for the northern hemispheric tropospheric columns while a small drift prevails for the period before 2011.

scholarly journals Estimating the Ice Crystal Enhancement Factor in the Tropics

2011 ◽  
Vol 68 (7) ◽  
pp. 1424-1434 ◽  
Author(s):  
Xiping Zeng ◽  
Wei-Kuo Tao ◽  
Toshihisa Matsui ◽  
Shaocheng Xie ◽  
Stephen Lang ◽  
...  
Keyword(s):  
Ice Crystal ◽  
Middle Latitudes ◽  
Ice Nuclei ◽  
Significant Difference ◽  
Physically Based ◽  
Cloud Resolving Model ◽  
The Difference ◽  
The Tropics ◽  
Cloud Condition

Abstract The ice crystal enhancement (IE) factor, defined as the ratio of the ice crystal to ice nuclei (IN) number concentrations for any particular cloud condition, is needed to quantify the contribution of changes in IN to global warming. However, the ensemble characteristics of IE are still unclear. In this paper, a representation of the IE factor is incorporated into a three-ice-category microphysical scheme for use in long-term cloud-resolving model (CRM) simulations. Model results are compared with remote sensing observations, which suggest that, absent a physically based consideration of how IE comes about, the IE factor in tropical clouds is about 103 times larger than that in midlatitudinal ones. This significant difference in IE between the tropics and middle latitudes is consistent with the observation of stronger entrainment and detrainment in the tropics. In addition, the difference also suggests that cloud microphysical parameterizations depend on spatial resolution (or subgrid turbulence parameterizations within CRMs).

scholarly journals Carbon and hydrogen isotopic ratios of atmospheric methane in the upper troposphere over the Western Pacific

2012 ◽  
Vol 12 (4) ◽  
pp. 9035-9077 ◽  
Author(s):  
T. Umezawa ◽  
T. Machida ◽  
K. Ishijima ◽  
H. Matsueda ◽  
Y. Sawa ◽  
...  
Keyword(s):  
Atmospheric Chemistry ◽  
Isotopic Ratio ◽  
Lower Troposphere ◽  
Western Pacific ◽  
Boreal Summer ◽  
Additional Contribution ◽  
Mixing Ratio ◽  
Upper Troposphere ◽  
The Tropics ◽  
The Western Pacific

Abstract. We present the mixing ratio, δ13C and δD of atmospheric CH4 using commercial aircraft in the upper troposphere (UT) over the Western Pacific for the period December 2005–September 2010. The observed results were compared with those obtained using commercial container ships in the lower troposphere (LT) over the same region. In the Northern Hemisphere (NH), the UT CH4 mixing ratio shows high values in the boreal summer–autumn, when the LT CH4 mixing ratio reaches a seasonal minimum. From tagged tracer experiments made using an atmospheric chemistry transport model, we found that such high CH4 values are due to rapid transport of air masses influenced by CH4 sources in South Asia and East Asia. The observed isotopic ratio data suggest that CH4 sources in these areas have relatively low δ13C and δD signatures, implying biogenic sources. Latitudinal distributions of the annual average UT and LT CH4 mixing ratio intersect each other in the tropics; the mixing ratio value is lower in the UT than in the LT in the NH and the situation is reversed in the Southern Hemisphere (SH), due mainly to the NH air intrusion into the SH through the UT. Such intersection of the latitudinal distributions is observable in δD but not in δ13C, implying additional contribution of a reaction of CH4 with active chlorine in the marine boundary layer. δ13C and δD show low values in the NH and high values in the SH both in the UT and in the LT. We also observed an increase in the CH4 mixing ratio and decreases in δ13C and δD during 2007–2008 in the UT and LT over the Western Pacific, possibly due to enhanced biogenic emissions in the tropics and NH.

scholarly journals Performance of the Vaisala RS80A/H and RS90 Humicap Sensors and the Meteolabor “Snow White” Chilled-Mirror Hygrometer in Paramaribo, Suriname

2006 ◽  
Vol 23 (11) ◽  
pp. 1506-1518 ◽  
Author(s):  
Gé Verver ◽  
Masatomo Fujiwara ◽  
Pier Dolmans ◽  
Cor Becker ◽  
Paul Fortuin ◽  
...  
Keyword(s):  
Relative Humidity ◽  
Time Lag ◽  
Lower Troposphere ◽  
Upper Troposphere ◽  
Weather Forecasts ◽  
Snow White ◽  
Study Results ◽  
The Tropics ◽  
Humidity Profiles ◽  
Dry Bias

Abstract In climate research there is a strong need for accurate observations of water vapor in the upper atmosphere. Radiosoundings provide relative humidity profiles but the accuracy of many routine instruments is notoriously inadequate in the cold upper troposphere. In this study results from a soundings program executed in Paramaribo, Suriname (5.8°N, 55.2°W), are presented. The aim of this program was to compare the performance of different humidity sensors in the upper troposphere in the Tropics and to test different bias corrections suggested in the literature. The payload of each sounding consisted of a chilled-mirror “Snow White” sensor from Meteolabor AG, which was used as a reference, and two additional sensors from Vaisala, that is, either the RS80A, the RS80H, or the RS90. In total 37 separate soundings were made. For the RS80A a clear, dry bias of between −4% and −8% RH is found in the lower troposphere compared to the Snow White observation, confirming the findings in previous studies. A mean dry bias was found in the upper troposphere, which could be effectively corrected. The RS80H sensor shows a significant wet bias of 2%–5% in RH in the middle and upper troposphere, which has not been reported before. Comparing observations with RS80H sensors of different ages gives no indication of sensor aging or sensor contamination. It is therefore concluded that the plastic cover introduced by Vaisala to avoid sensor contamination is effective. Finally, the RS90 sensor yields a small but significant wet bias of 2%–3% below 7-km altitude. The time-lag error correction from Miloshevich et al. was applied to the Vaisala data, which resulted in an increased variability in the relative humidity profile above 9- (RS80A), 8- (RS80H), and 11-km (RS90) altitude, respectively, which is in better agreement with the Snow White data. The averaged Snow White profile is compared with the average profiles of relative humidity from the European Centre for Medium-Range Weather Forecasts (ECMWF). No significant bias is found in either the analyses or the forecasts. The correlation coefficient for the Snow White and ECMWF data between 200 and 800 hPa was 0.66 for the 36-h forecast and 0.77 for the analysis.

scholarly journals Characterization of ozone profiles derived from Aura TES and OMI Radiances

2012 ◽  
Vol 12 (10) ◽  
pp. 27589-27636 ◽  
Author(s):  
D. Fu ◽  
J. R. Worden ◽  
X. Liu ◽  
S. S. Kulawik ◽  
K. W. Bowman ◽  
...  
Keyword(s):  
Degrees Of Freedom ◽  
Surface Ozone ◽  
Lower Troposphere ◽  
Vertical Resolution ◽  
Ozone Monitoring Instrument ◽  
Near Surface ◽  
Upper Troposphere ◽  
Ozone Profile ◽  
Mean Square Difference

Abstract. We present satellite based ozone profile estimates derived by combining radiances measured at thermal infrared (TIR) wavelengths from the Aura Tropospheric Emission Spectrometer (TES) and ultraviolet (UV) wavelengths measured by the Aura Ozone Monitoring Instrument (OMI). The advantage of using these combined wavelengths and instruments for sounding ozone over either instrument alone is improved sensitivity near the surface as well as the capability to consistently resolve the lower troposphere, upper troposphere, and lower stratosphere for scenes with varying geophysical states. For example, the vertical resolution for ozone estimates from either TES or OMI vary strongly by surface albedo and temperature and typically provide 1.6 degrees-of-freedom for signal (DOFS) for TES or less than 1 DOFS for OMI in the troposphere. The combination typically provides 2 degrees-of-freedom for signal (DOFS) in the troposphere with approximately 0.4 DOFS for near surface ozone (surface to 700 hPa). We evaluate these new ozone profile estimates with ozonesonde measurements and find that calculated errors for the joint TES and OMI ozone profile estimates are in approximate agreement with actual errors as derived by the root-mean-square difference between the ozonesondes and the joint TES/OMI ozone estimates. We find that the vertical resolution of the joint TES/OMI ozone profile estimate is sufficient for quantifying variations in near-surface ozone with a precision of 26% (15.6 ppb) and a bias of 9.6% (5.7 ppb).

scholarly journals Global large-scale stratosphere-troposphere exchange in modern reanalyses

2016 ◽  
Author(s):  
Alexander C. Boothe ◽  
Cameron R. Homeyer
Keyword(s):  
Large Scale ◽  
Lower Stratosphere ◽  
Radiative Properties ◽  
Lapse Rate ◽  
Polar Regions ◽  
Transport Mechanisms ◽  
Upper Troposphere ◽  
Long Term Changes ◽  
The Tropics

Abstract. Stratosphere-troposphere exchange (STE) has important and significant impacts on the chemical and radiative properties of the upper troposphere and lower stratosphere. This study presents a 15-year climatology of global large-scale STE from four modern reanalyses: ERA-Interim, JRA-55, MERRA-2, and MERRA-1. STE is separated into four categories for analysis to identify the significance of known transport mechanisms: 1) vertical stratosphere-to-troposphere transport (STT), 2) vertical troposphere-to-stratosphere transport (TST), 3) lateral STT (that occurring between the tropics and the extratropics and across the tropopause "break"), and 4) lateral TST. In addition, this study employs a method to identify STE as that which crosses the lapse-rate tropopause (LRT), while most previous studies have used a potential vorticity (PV) isosurface as the troposphere-stratosphere boundary. PV-based and LRT based STE climatologies are compared using the same reanalysis output (ERA-Interim). The comparison reveals quantitative and qualitative differences, particularly in the geographic representation of TST in the polar regions. Based upon spatiotemporal integrations, we find STE to be STT-dominant in ERA-Interim and JRA-55 and TST-dominant in the MERRA reanalyses. Time series during the 15-year analysis period show long-term changes that are argued to correspond with changes in the Brewer-Dobson circulation.

The World Food Conference

2017 ◽  
Author(s):  
Barry Riley
Keyword(s):  
The United States ◽  
Food Prices ◽  
Food Aid ◽  
World Food ◽  
High Food ◽  
White House ◽  
The World ◽  
The Difference ◽  
Global Food

Just before leaving the White House to assume his duties as secretary of state, Kissinger alerted top Agriculture officials in Washington that the president was increasingly concerned with the growing world food crisis. Among the responses was word that the American food aid program was not going to be able to meet its global food aid commitments because of the combination of high food prices and budgetary constraints. Shortly thereafter Kissinger publicly called for the convening of a World Food Conference to consider the problem and propose long-term remedies. This chapter describes interagency debates over what the United States should—and should not—promise in the conference. It highlights the difference between domestic agriculture interests, represented by Secretary of Agriculture Butz, foreign policy interests, exemplified by Kissinger, humanitarian concerns, voiced by Senator Humphrey, and the perspective of the new president, Gerald Ford.

scholarly journals Global large-scale stratosphere–troposphere exchange in modern reanalyses

2017 ◽  
Vol 17 (9) ◽  
pp. 5537-5559 ◽  
Author(s):  
Alexander C. Boothe ◽  
Cameron R. Homeyer
Keyword(s):  
Large Scale ◽  
Lower Stratosphere ◽  
Radiative Properties ◽  
Lapse Rate ◽  
Polar Regions ◽  
Transport Mechanisms ◽  
Upper Troposphere ◽  
Subtropical Jet ◽  
The Tropics

Abstract. Stratosphere–troposphere exchange (STE) has important impacts on the chemical and radiative properties of the upper troposphere and lower stratosphere. This study presents a 15-year climatology of global large-scale STE from four modern reanalyses: ERA-Interim, JRA-55, MERRA-2, and MERRA. STE is separated into three regions (tropics, subtropics, and extratropics) and two transport directions (stratosphere-to-troposphere transport or STT and troposphere-to-stratosphere transport or TST) in an attempt to identify the significance of known transport mechanisms. The extratropics and tropics are separated by the tropopause break. Any STE occurring between the tropics and the extratropics through the tropopause break is considered subtropical exchange (i.e., in the vicinity of the subtropical jet). In addition, this study employs a method to identify STE as that which crosses the lapse-rate tropopause (LRT), while most previous studies have used a potential vorticity (PV) isosurface as the troposphere–stratosphere boundary. PV-based and LRT-based STE climatologies are compared using the ERA-Interim reanalysis output. The comparison reveals quantitative and qualitative differences, particularly for TST in the polar regions. Based upon spatiotemporal integrations, we find STE to be STT dominant in ERA-Interim and JRA-55 and TST dominant in MERRA and MERRA-2. The sources of the differences are mainly attributed to inconsistencies in the representation of STE in the subtropics and extratropics. Time series during the 15-year analysis period show long-term changes that are argued to correspond with changes in the Brewer–Dobson circulation.

scholarly journals The Downward Influence of Sudden Stratospheric Warmings: Association with Tropospheric Precursors

2018 ◽  
Vol 32 (1) ◽  
pp. 85-108 ◽  
Author(s):  
Ian White ◽  
Chaim I. Garfinkel ◽  
Edwin P. Gerber ◽  
Martin Jucker ◽  
Valentina Aquila ◽  
...  
Keyword(s):  
Climate Model ◽  
Lower Troposphere ◽  
Wave Activity ◽  
Extreme Wave ◽  
Northern Annular Mode ◽  
Downward Influence ◽  
The Difference ◽  
The Relationship ◽  
Barotropic Response

AbstractTropospheric features preceding sudden stratospheric warming events (SSWs) are identified using a large compendium of events obtained from a chemistry–climate model. In agreement with recent observational studies, it is found that approximately one-third of SSWs are preceded by extreme episodes of wave activity in the lower troposphere. The relationship becomes stronger in the lower stratosphere, where ~60% of SSWs are preceded by extreme wave activity at 100 hPa. Additional analysis characterizes events that do or do not appear to subsequently impact the troposphere, referred to as downward and non-downward propagating SSWs, respectively. On average, tropospheric wave activity is larger preceding downward-propagating SSWs compared to non-downward propagating events, and associated in particular with a doubly strengthened Siberian high. Of the SSWs that were preceded by extreme lower-tropospheric wave activity, ~2/3 propagated down to the troposphere, and hence the presence of extreme lower-tropospheric wave activity can only be used probabilistically to predict a slight increase or decrease at the onset, of the likelihood of tropospheric impacts to follow. However, a large number of downward and non-downward propagating SSWs must be considered (>35), before the difference becomes statistically significant. The precursors are also robust upon comparison with composites consisting of randomly selected tropospheric northern annular mode (NAM) events. The downward influence and precursors to split and displacement events are also examined. It is found that anomalous upward wave-1 fluxes precede both cases. Splits exhibit a near instantaneous, barotropic response in the stratosphere and troposphere, while displacements have a stronger long-term influence.

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