scholarly journals Refinement of the ice absorption spectrum in the visible using radiance profile measurements in Antarctic snow

2016 ◽  
Author(s):  
Ghislain Picard ◽  
Quentin Libois ◽  
Laurent Arnaud

Abstract. Ice is a highly transparent material in the visible. According to the most widely used database (Warren and Brandt, 2008; IA2008), the ice absorption coefficient reaches values lower than 10−3 m−1 around 400 nm. These values were obtained from a radiance profile measured in a single snow layer at Dome C in Antarctica. We reproduced this experiment using a fiber optics inserted in the snow to record 56 profiles from which 70 homogeneous layers were identified. Applying the same estimation method on every layer yields 70 ice absorption spectra with a significant variability and overall larger than IA2008 by one order of magnitude. We devise another estimation method based on Bayesian inference. It reduces the statistical variability and confirms the higher absorption, around 2 × 10−2 m−1 near the minimum at 440 nm. We explore potential instrumental artifacts by developing a 3D radiative transfer model able to explicitly account for the presence of the fiber in the snow. The simulation results show that the radiance profile is indeed perturbed by the fiber intrusion but the error on the ice absorption estimate is not larger than a factor 2. This is insufficient to explain the difference between our new estimate and IA2008. Nevertheless, considering the number of profiles acquired for this study and other estimates from the Antarctic Muon and Neutrino Detector Array (AMANDA), we estimate that ice absorption values around 10−2 m−1 at the minimum are more likely than under 10−3 m−1. We provide a new estimate in the range 400–600 nm for future modeling of snow, cloud, and sea-ice optical properties. Most importantly we recommend that modeling studies take into account the large uncertainty of the ice absorption coefficient in the visible.

2016 ◽  
Vol 10 (6) ◽  
pp. 2655-2672 ◽  
Author(s):  
Ghislain Picard ◽  
Quentin Libois ◽  
Laurent Arnaud

Abstract. Ice is a highly transparent material in the visible. According to the most widely used database (IA2008; Warren and Brandt, 2008), the ice absorption coefficient reaches values lower than 10−3 m−1 around 400 nm. These values were obtained from a vertical profile of spectral radiance measured in a single snow layer at Dome C in Antarctica. We reproduced this experiment using an optical fiber inserted in the snow to record 56 profiles from which 70 homogeneous layers were identified. Applying the same estimation method on every layer yields 70 ice absorption spectra. They present a significant variability but absorption coefficients are overall larger than IA2008 by 1 order of magnitude at 400–450 nm. We devised another estimation method based on Bayesian inference that treats all the profiles simultaneously. It reduces the statistical variability and confirms the higher absorption, around 2  ×  10−2 m−1 near the minimum at 440 nm. We explore potential instrumental artifacts by developing a 3-D radiative transfer model able to explicitly account for the presence of the fiber in the snow. The simulation shows that the radiance profile is indeed perturbed by the fiber intrusion, but the error on the ice absorption estimate is not larger than a factor of 2. This is insufficient to explain the difference between our new estimate and IA2008. The same conclusion applies regarding the plausible contamination by black carbon or dust, concentrations reported in the literature are insufficient. Considering the large number of profiles acquired for this study and other estimates from the Antarctic Muon and Neutrino Detector Array (AMANDA), we nevertheless estimate that ice absorption values around 10−2 m−1 at the minimum are more likely than under 10−3 m−1. A new estimate in the range 400–600 nm is provided for future modeling of snow, cloud, and sea-ice optical properties. Most importantly, we recommend that modeling studies take into account the large uncertainty of the ice absorption coefficient in the visible and that future estimations of the ice absorption coefficient should also thoroughly account for the impact of the measurement method.


2021 ◽  
Vol 13 (11) ◽  
pp. 2061
Author(s):  
Mikhail V. Belikovich ◽  
Mikhail Yu. Kulikov ◽  
Dmitry S. Makarov ◽  
Natalya K. Skalyga ◽  
Vitaly G. Ryskin ◽  
...  

Ground-based microwave radiometers are increasingly used in operational meteorology and nowcasting. These instruments continuously measure the spectra of downwelling atmospheric radiation in the range 20–60 GHz used for the retrieval of tropospheric temperature and water vapor profiles. Spectroscopic uncertainty is an important part of the retrieval error budget, as it leads to systematic bias. In this study, we analyze the difference between observed and simulated microwave spectra obtained from more than four years of microwave and radiosonde observations over Nizhny Novgorod (56.2° N, 44° E). We focus on zenith-measured and elevation-scanning data in clear-sky conditions. The simulated spectra are calculated by a radiative transfer model with the use of radiosonde profiles and different absorption models, corresponding to the latest spectroscopy research. In the case of zenith-measurements, we found a systematic bias (up to ~2 K) of simulated spectra at 51–54 GHz. The sign of bias depends on the absorption model. A thorough investigation of the error budget points to a spectroscopic nature of the observed differences. The dependence of the results on the elevation angle and absorption model can be explained by the basic properties of radiative transfer and by cloud contamination at elevation angles.


2016 ◽  
Vol 9 (8) ◽  
pp. 2741-2754 ◽  
Author(s):  
Elham Baranizadeh ◽  
Benjamin N. Murphy ◽  
Jan Julin ◽  
Saeed Falahat ◽  
Carly L. Reddington ◽  
...  

Abstract. The particle formation scheme within PMCAMx-UF, a three-dimensional chemical transport model, was updated with particle formation rates for the ternary H2SO4–NH3–H2O pathway simulated by the Atmospheric Cluster Dynamics Code (ACDC) using quantum chemical input data. The model was applied over Europe for May 2008, during which the EUCAARI-LONGREX (European Aerosol Cloud Climate and Air Quality Interactions–Long-Range Experiment) campaign was carried out, providing aircraft vertical profiles of aerosol number concentrations. The updated model reproduces the observed number concentrations of particles larger than 4 nm within 1 order of magnitude throughout the atmospheric column. This agreement is encouraging considering the fact that no semi-empirical fitting was needed to obtain realistic particle formation rates. The cloud adjustment scheme for modifying the photolysis rate profiles within PMCAMx-UF was also updated with the TUV (Tropospheric Ultraviolet and Visible) radiative-transfer model. Results show that, although the effect of the new cloud adjustment scheme on total number concentrations is small, enhanced new-particle formation is predicted near cloudy regions. This is due to the enhanced radiation above and in the vicinity of the clouds, which in turn leads to higher production of sulfuric acid. The sensitivity of the results to including emissions from natural sources is also discussed.


Author(s):  
H. Lin ◽  
X. Zhang ◽  
Y. Yang ◽  
X. Wu ◽  
D. Guo

From geologic perspective, understanding the types, abundance, and size distributions of minerals allows us to address what geologic processes have been active on the lunar and planetary surface. The imaging spectrometer which was carried by the Yutu Rover of Chinese Chang’E-3 mission collected the reflectance at four different sites at the height of ~ 1 m, providing a new insight to understand the lunar surface. The mineral composition and Particle Size Distribution (PSD) of these four sites were derived in this study using a Radiative Transfer Model (RTM) and Sparse Unmixing (SU) algorithm. The endmembers used were clinopyroxene, orthopyroxene, olivine, plagioclase and agglutinate collected from the lunar sample spectral dataset in RELAB. The results show that the agglutinate, clinopyroxene and olivine are the dominant minerals around the landing site. In location Node E, the abundance of agglutinate can reach up to 70 %, and the abundances of clinopyroxene and olivine are around 10 %. The mean particle sizes and the deviations of these endmembers were retrieved. PSDs of all these endmembers are close to normal distribution, and differences exist in the mean particle sizes, indicating the difference of space weathering rate of these endmembers.


2007 ◽  
Vol 46 ◽  
pp. 375-381 ◽  
Author(s):  
Teruo Aoki ◽  
Hiroki Motoyoshi ◽  
Yuji Kodama ◽  
Teppei J. Yasunari ◽  
Konosuke Sugiura

AbstractContinuous measurements of the radiation budget and meteorological components, along with frequent snow-pit work, were performed in Sapporo, Hokkaido, Japan, during two winters from 2003 to 2005. The measured relationships between broadband albedos and the mass concentration of snow impurities were compared with theoretically predicted relationships calculated using a radiative transfer model for the atmosphere–snow system in which different types (in light absorption) of impurity models based on mineral dust and soot were assumed. The result suggests that the snow in Sapporo was contaminated not only with mineral dust but also with more absorptive soot. A comparison of the measured relationships between broadband albedos and snow grain size for two different layers with the theoretically predicted relationships revealed that the visible albedo contains information about the snow grain size in deeper snow layers (10 cm), and the near-infrared albedo contains only surface information. This is due to the difference in penetration depth of solar radiation into snow between the visible and the near-infrared wavelengths.


2018 ◽  
Vol 11 (7) ◽  
pp. 2763-2788 ◽  
Author(s):  
Ghislain Picard ◽  
Melody Sandells ◽  
Henning Löwe

Abstract. The Snow Microwave Radiative Transfer (SMRT) thermal emission and backscatter model was developed to determine uncertainties in forward modeling through intercomparison of different model ingredients. The model differs from established models by the high degree of flexibility in switching between different electromagnetic theories, representations of snow microstructure, and other modules involved in various calculation steps. SMRT v1.0 includes the dense media radiative transfer theory (DMRT), the improved Born approximation (IBA), and independent Rayleigh scatterers to compute the intrinsic electromagnetic properties of a snow layer. In the case of IBA, five different formulations of the autocorrelation function to describe the snow microstructure characteristics are available, including the sticky hard sphere model, for which close equivalence between the IBA and DMRT theories has been shown here. Validation is demonstrated against established theories and models. SMRT was used to identify that several former studies conducting simulations with in situ measured snow properties are now comparable and moreover appear to be quantitatively nearly equivalent. This study also proves that a third parameter is needed in addition to density and specific surface area to characterize the microstructure. The paper provides a comprehensive description of the mathematical basis of SMRT and its numerical implementation in Python. Modularity supports model extensions foreseen in future versions comprising other media (e.g., sea ice, frozen lakes), different scattering theories, rough surface models, or new microstructure models.


2019 ◽  
Vol 11 (19) ◽  
pp. 2240 ◽  
Author(s):  
David Santek ◽  
Richard Dworak ◽  
Sharon Nebuda ◽  
Steve Wanzong ◽  
Régis Borde ◽  
...  

Atmospheric Motion Vectors (AMVs) calculated by six different institutions (Brazil Center for Weather Prediction and Climate Studies/CPTEC/INPE, European Organization for the Exploitation of Meteorological Satellites/EUMETSAT, Japan Meteorological Agency/JMA, Korea Meteorological Administration/KMA, Unites States National Oceanic and Atmospheric Administration/NOAA, and the Satellite Application Facility on Support to Nowcasting and Very short range forecasting/NWCSAF) with JMA’s Himawari-8 satellite data and other common input data are here compared. The comparison is based on two different AMV input datasets, calculated with two different image triplets for 21 July 2016, and the use of a prescribed and a specific configuration. The main results of the study are summarized as follows: (1) the differences in the AMV datasets depend very much on the ‘AMV height assignment’ used and much less on the use of a prescribed or specific configuration; (2) the use of the ‘Common Quality Indicator (CQI)’ has a quantified skill in filtering collocated AMVs for an improved statistical agreement between centers; (3) Among the six AMV operational algorithms verified by this AMV Intercomparison, JMA AMV algorithm has the best overall performance considering all validation metrics, mainly due to its new height assignment method: ‘Optimal estimation method considering the observed infrared radiances, the vertical profile of the Numerical Weather Prediction wind, and the estimated brightness temperature using a radiative transfer model’.


2014 ◽  
Vol 14 (6) ◽  
pp. 2987-3015 ◽  
Author(s):  
C. S. Zerefos ◽  
P. Tetsis ◽  
A. Kazantzidis ◽  
V. Amiridis ◽  
S. C. Zerefos ◽  
...  

Abstract. We examine sunsets painted by famous artists as proxy information for the aerosol optical depth after major volcanic eruptions. Images derived from precision colour protocols applied to the paintings were compared to online images, and found that the latter, previously analysed, provide accurate information. Aerosol optical depths (AODs) at 550 nm, corresponding to Northern Hemisphere middle latitudes, calculated by introducing red-to-green (R / G) ratios from a large number of paintings to a radiative transfer model, were significantly correlated with independent proxies from stratospheric AOD and optical extinction data, the dust veil index, and ice core volcanic indices. AODs calculated from paintings were grouped into 50-year intervals from 1500 to 2000. The year of each eruption and the 3 following years were defined as "volcanic". The remaining "non-volcanic" years were used to provide additional evidence of a multidecadal increase in the atmospheric optical depths during the industrial "revolution". The increase of AOD at 550 nm calculated from the paintings grows from 0.15 in the middle 19th century to about 0.20 by the end of the 20th century. To corroborate our findings, an experiment was designed in which a master painter/colourist painted successive sunsets during and after the passage of Saharan aerosols over the island of Hydra in Greece. Independent solar radiometric measurements confirmed that the master colourist's R / G ratios which were used to model his AODs, matched the AOD values measured in situ by co-located sun photometers during the declining phase of the Saharan aerosol. An independent experiment was performed to understand the difference between R / G ratios calculated from a typical volcanic aerosol and those measured from the mineral aerosol during the Hydra experiment. It was found that the differences in terms of R / G ratios were small, ranging between −2.6% and +1.6%. Also, when analysing different parts of cloudless skies of paintings following major volcanic eruptions, any structural differences seen in the paintings had not altered the results discussed above. However, a detailed study on all possible sources of uncertainties involved (such as the impact of clouds on R / G ratios) still needs to be studied. Because of the large number of paintings studied, we tentatively propose the conclusion that regardless of the school, red-to-green ratios from great masters can provide independent proxy AODs that correlate with widely accepted proxies and with independent measurements.


2008 ◽  
Vol 4 (S252) ◽  
pp. 263-264
Author(s):  
Huan Wang ◽  
B. W. Jiang ◽  
R. Szczerba

AbstractWith the Mie theory and the radiative transfer model, we studied the effect of dust size on the infrared color indexes concerning special filters used in the space infrared missions and typical filters in the near-infrared, of AGB stars with typical oxygen-rich and carbon-rich dust shells. It is found the most affected bands are the near-infrared bands JHK and the Spitzer IRAC bands, meanwhile the wavebands with reference wavelength longer than 10 μm is little affected. The effect increases fast with the mass loss rate. We also discussed the potential to distinguish the O-rich and C-rich dusts, and the difference in IR colors between the AGB stars and other IR sources like YSOs and galaxies.


2016 ◽  
Vol 7 ◽  
pp. 2037-2044 ◽  
Author(s):  
Aparna Zagabathuni ◽  
Sudipto Ghosh ◽  
Shyamal Kumar Pabi

A suspension of particles below 100 nm in size, usually termed as nanofluid, often shows a notable enhancement in thermal conductivity, when measured by the transient hot-wire method. In contrast, when the conductivity of the same nanofluid is measured by the laser flash method, the enhancement reported is about one order of magnitude lower. This difference has been quantitatively resolved for the first time on the basis of the collision-mediated heat transfer model for nanofluids proposed earlier by our research group. Based on the continuum simulation coupled with stochastic analysis, the present theoretical prediction agrees well with the experimental observations from different measuring methods reported in the literature, and fully accounts for the different results from the two measuring methods mentioned above. This analysis also gives an indication that the nanofluids are unlikely to be effective for heat transfer in microchannels.


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