Femtosecond pumping of nuclear isomeric states by the Coulomb collision of ions with quivering electrons
Abstract Efficient production of metastable quantum states of nuclei (isomers) is critical for exotic applica- tions, like nuclear clocks, nuclear batteries, clean nuclear energy, and nuclear gamma-ray lasers[1–6]. However, due to low reaction cross sections and quick decay, it is extremely difficult to acquire sig- nificant amount of isomers with short lifetimes via traditional accelerators or reactors. Here, we present femtosecond pumping of nuclear isomeric states by the Coulomb excitation of ions with the quivering electrons induced by laser fields for the first time. Nuclear isomers populated on the second excited state of 83Kr, are generated with a rate of 3.84 × 10^17 per second from a table-top hundreds-TW laser system. This high efficiency of isomer production can be explained by Coulomb collision[7] of ions with the quivering electrons during the laser-cluster interactions at nearly solid densities.